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作 者:Danni Xie Xiaodong Ge Lei Duan Jan Mulder
机构地区:[1]School of Land Engineering,Chang’an University,Xi’an 710064,China [2]State Key Laboratory of Environmental Simulation and Pollution Control,School of Environment,Tsinghua University,Beijing 100084,China [3]State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex,Beijing 100084,China [4]Faculty of Environmental Sciences and Natural Resource Management,Norwegian University of Life Sciences,Box 5003,NO-1432,Ås,Norway
出 处:《Frontiers of Environmental Science & Engineering》2024年第6期115-126,共12页环境科学与工程前沿(英文)
基 金:the National Key Research and Development Project(No.2022YFC3700600);the National Natural Science Foundation of China(Nos.42303061 and 42277204);the Norwegian Directorate for Higher Education and Skills(HK-DIR,projects UTF-2016-long-term/10089 and UTF-2020/10180);the Young Talent Fund of Association for Science and Technology in Shaanxi,China(20230704).
摘 要:For many decades,acid deposition used to pose a significant regional air pollution challenge in China.After substantial emission control of anthropogenically derived sulfur and nitrogen containing gasses,both sulfur and nitrogen deposition,as well as the acid rain-affected area,have significantly decreased compared to their peak levels.Forests,particularly in the humid subtropics,are sensitive to acid deposition,as evidenced by soil acidification,sulfate and nitrate leaching in stream water,and elevated soil nitrous oxide emission.Reduction in the total deposition of sulfur and nitrogen,caused a significant decline in sulfate and nitrate leaching from subtropical forest and subsequently in sulfate and nitrate concentrations in stream water,although there was about a 5-year delay.This delay may be attributed to the desorption of accumulated sulfate and continued elevated mineralization of accumulated nitrogen pools.Emissions of nitrous oxide,a potent greenhouse gas,also declined in nitrogen-saturated subtropical forest soils,as soil water nitrate concentration decreased.Therefore,subtropical forests in China suffering from elevated acid deposition have begun to recover.Yet,the current levels of sulfur and nitrogen deposition continue to exceed the critical loads,i.e.,the assigned threshold levels in accordance with emission control policies,in more than 10%of the country’s land area,respectively,indicating remaining risks of acidification and eutrophication.Thus,further emission reductions are urgently needed,also because they will help achieving goals related to air quality and nitrous oxide emissions.
关 键 词:ACIDIFICATION Critical load Nitrous oxide Surface water chemistry RECOVERY
分 类 号:X53[环境科学与工程—环境工程]
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