THIOLATE

作品数：44被引量：14H指数：2
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Single thiolate replacement of metal nanoclusters
《Science China Chemistry》2024年第2期523-528,共6页Ambreen Ambreen Yue Zhou Wanmiao Gu Qing You Liang Fang Guoqing Bian Nan Yan Nan Xia Zhikun Wu 
supported by the National Natural Science Foundation of China (21925303,21829501,21771186,22171268,22171267,21971246);the Anhui Provincial Natural Science Foundation(2108085MB56);the HFIPS Director’s Fund (BJPY2019A02,YZJJ202102,YZJJ202306-TS);the Collaborative Innovation Program of Hefei Science Center,Chinese Academy of Sciences (2020HSC-CIP005,2022HSCCIP018)。
Surface thiolates play important roles in evincing the structures and properties of thiolated metal nanoclusters—one type of recently emerging inorganic-organic hybrids,and thus the thiolate substitution,especially s...
关键词：metal nanoclusters single thiolate replacement thermal expansion STABILITY intercluster interaction 
Bulky Thiolate-Protected Silver Nanocluster Ag_(213)(Adm-S)_(44)Cl_(33)with Excellent Electrocatalytic Performance toward Oxygen Reduction
《CCS Chemistry》2023年第5期1154-1162,共9页Chen-Guang Shi Jian-Hua Jia Yaling Jia Guangqin Li Ming-Liang Tong 
supported by the National Natural Science Foundation of China(grant nos.21771198,22071274,21821003).
Atomically precise gold and/or silver nanoclusters play a key role in crystallography and coordination chemistry.Compared with gold nanoclusters,silver nanoclusters become unstable and difficult to crystallize due to ...
关键词：SILVER NANOCLUSTERS atomically precise structure oxygen reduction reaction electrocatalysis 
Atomically precise thiolate-protected gold nanoclusters:Current status of designability of the structure and physicochemical properties
《Aggregate》2023年第2期1-41,共41页Sakiat Hossain Daisuke Hirayama Ayaka Ikeda Mai Ishimi Sota Funaki Arpan Samanta Tokuhisa Kawawaki Yuichi Negishi 
Japan Society for the Promotion of Science,Grant/Award Numbers:20H02698,20H02552,18H05178,20H05115;Hydrogenomics,Grant/Award Number:21H00027;Aquatic Functional Materials,Grant/Award Numbers:18H05178,22H04562;Yazaki Memorial Foundation for Science and Technology;Ogasawara Foundation for the Promotion of Science and Engineering;Kao Foundation for Arts and Sciences;TEPCO Memorial Foundation;Japan Science Society;Takahashi Industrial and Economic Research Foundation;Kubota Corporation。
Thiolate(SR)-protected gold nanoclusters(Aun(SR)m NCs)are a rare type of material capable of simultaneously exhibiting multiple physicochemical properties well-suited to specific applications,including photoluminescen...
关键词：atomically precise metal nanoclusters gold nanoclusters physicochemical properties STRUCTURES THIOLATE 
The 3,4-dimethoxybenzyl group as solubilizing protective group for the in situ deprotection/deposition of extended aromatic thiolate monolayers
《Nano Research》2023年第1期1695-1702,共8页Adrian Wiesner Sonja Katzbach Dariusz Bebej Martina Dettenhöfer Michael Zharnikov Andreas Terfort 
While self-assembled monolayers(SAMs)of aromatic thiolates are frequently used in a wide range of applications,their formation is often hampered by the low solubilities of their precursors.Here we introduce the 3,4-di...
关键词：self-assembled monolayers protective group SOLUBILITY scanning-tunneling microscopy infrared-reflection absorption spectroscopy 
A Low-Crossover and Fast-Kinetics Thiolate Negolyte for Aqueous Redox Flow Batteries被引量：2
《Energy Material Advances》2022年第1期377-387,共11页Bin Yang Zengyue Wang Wanwan Wang Yi-Chun Lu 
This work is supported by grants from the Research Grants Council(RGC)of the Hong Kong Administrative Region,China,under a RGC project no.T23-601/17-R.
Aqueous redox flow batteries(ARFBs)are a promising technology for large-scale energy storage.Developing high-capacity and long-cycle negolyte materials is one of major challenges for practical ARFBs.Inorganic polysulf...
关键词：SULFIDE KINETICS CROSSOVER 
Temperature-dependent chloride-mediated access to atom-precise silver thiolate nanoclusters被引量：2
《Science China Chemistry》2022年第6期1094-1099,共6页Ling Yang Xin-Yao Wang Xiao-Yan Tang Meng-Yi Wang Chun-Yan Ni Hong Yu Ying-Lin Song Brendan F.Abrahams Jian-Ping Lang 
supported by the National Natural Science Foundation of China (21871196, 21773163, 21531006);the Collaborative Innovation Center of Suzhou Nano Science and Technology;the Priority Academic Program Development of Jiangsu Higher Education Institutions;the Project of Scientific and Technologic Infrastructure of Suzhou (SZS201905)。
By using a unique temperature-dependent,chloride-mediated approach,two atom-precise silver nanoclusters[Cl@Ag_(14)(Tab)_(12)-(C_(5)H_(4)NCl)_(12)](PF_(6))_(13)(Cl@Ag_(14))and[Cl_(3)@Ag_(24)(Tab)_(20)(C_(5)H_(4)NCl)_(1...
关键词：TEMPERATURE-DEPENDENT chloride-mediated core expansion silver thiolate nanocluster transformation 
Construction of a low-valent thiolate-bridged dicobalt platform and its reactivity toward hydrogen activation and evolution
《Chinese Chemical Letters》2022年第5期2477-2480,共4页Tao Mei Dawei Yang Linan Su Baomin Wang Jingping Qu 
supported by the National Natural Science Foun-dation of China(Nos.21690064,22001031);Key Laboratory of Bio-based Chemicals of Liaoning Province of China,the“111”project of the Ministry of Education of China and the Fundamental Research Funds for the Central Universities(No.DUT19RC(3)013).
Low-valence transition metallic complexes have drawn longstanding attention due to their high reactivity toward catalytic transformation of various small molecules.Among these known complexes,the low-valence metal cen...
关键词：Low-valence Thiolate-bridged Cobalt Homolytic H_(2)cleavage HYDRIDE Hydrogen evolution 
Anion-templated Self-assembly for the Preparation of Silver-t-butylthiolate Clusters被引量：1
《Chinese Journal of Structural Chemistry》2022年第3期100-107,I0010,共9页JIN Jun-Ling SHEN Yang-Lin MI Li-Wei XIE Yun-Peng LU Xing 
supported by the National Natural Science Foundation of China (No. 21771071, 22171094, and 21925104);the Key Scientific Research Projects of Universities in Henan Province (No. 21A150060)
Silver thiolate polymers are intercepted to form different structural fragments when reacting with variant solubilizing reagents,which usually serve as the starting point for the preparation of clusters.However,such a...
关键词：silver cluster X-ray crystal structure silver thiolate polymer SELF-ASSEMBLY 
Interfaced Ag/Cu nanostructures derived from metal thiolate nanoplates:A highly selective catalyst for electrochemical reduction of CO_(2) to ethanol
《SmartMat》2022年第1期173-182,共10页Sasitha C.Abeyweera Matas Simukaitis Qilin Wei Yugang Sun 
Selective reduction of CO_(2) into liquid products such as ethanol through electrochemical catalysis is promising in storing renewable energy in more deliverable chemicals and balancing the carbon footprint in the env...
关键词：carbon dioxide to liquid fuels electrical‐to‐chemical energy conversion interfaced bimetallic boundaries C-C coupling reactions 
Synthesis,characterization and reactivity of thiolate-bridged cobalt-iron and ruthenium-iron complexes
《Chinese Chemical Letters》2022年第1期217-220,共4页Chao Guo Linan Su Dawei Yang Baomin Wang Jingping Qu 
supported by the National Natural Science Foundation of China(Nos.21690064,22001031);the key laboratory of Bio-based Chemicals of Liaoning Province of China;the“111”project of the Ministry of Education of China;the Fundamental Research Funds for the Central Universities(No.DUT19RC(3)013)。
Thiolate-bridged hetero-bimetallic complexes[Cp^(*)M(MeCN)N_(2)S_(2)FeCl][PF_(6)](2,M=Ru;3,M=Co,Cp^(*)=η^(5)-C_(5)Me_(5),N_(2)S_(2)=N,N'-dimethyl-3,6-diazanonane-1,8-dithiolate)were prepared by self-assembly of dimer...
关键词：Metallic cooperativity Heterobinuclear complex Hydrazine disproportionation Metallothiolate ligand Metal-sulfur cluster 
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