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Silicalite-1 zeolite nanosheets with rich H-bonded silanols for boosting vapor-phase Beckmann rearrangement:One-pot synthesis and theoretical investigation
《Chinese Journal of Catalysis》2024年第12期82-90,共9页Tianming Zai Wei Chen Jiamin Yuan Ye Ma Qinming Wu Xianfeng Yi Zhiqiang Liu Xiangju Meng Weiliao Liu Na Sheng Han Wang Anmin Zheng Feng-Shou Xiao 
国家自然科学基金(22288101,22172141);浙江省自然科学基金(LR24B030001);武汉市自然科学基金(2024040701010058).
Design and preparation of highly efficient zeolite catalysts for gas-phase Beckmann rearrangement of cyclohexanone oxime to caprolactam are attractive but still challenging.Herein,we show a one-pot synthesis of silica...
关键词:Silicalite-1 zeolite nanosheets Rich H-bonded silanols One-pot synthesis Vapor-phase Beckmann rearrangement Theoretical investigation 
Expired drugs as vapor-phase corrosion inhibitors of copper in simulated marine atmospheric environment
《Journal of Central South University》2024年第10期3570-3582,共13页WANG Xin-wei ZHANG Tian-long LI Yan-tao YANG Li-hui XU Wei-chen DISNA Ratnasekera HAN Tao 
Project(ZR2023ME063)supported by the Shandong Provincial Natural Science Foundation,China;Project(121311KYSB20210005)supported by the Overseas Science and Education Cooperation Center Deployment Project,China;Project supported by the Qingdao Expert Workstation for Intelligent Anticorrosion for Water Diversion Project,China。
Urea,paracetamol and glutamine(based on the expired drugs)were selected as vapor-phase corrosion inhibitors(VCIs)to study their corrosion protection effect on red copper in simulated marine atmospheric environment by ...
关键词:marine corrosion and protection vapor-phase corrosion inhibitor(VCI) COPPER expired drugs marine atmospheric environment 
Vapor-phase postsynthetic amination of hypercrosslinked polymers for efficient iodine capture被引量:1
《Chinese Chemical Letters》2024年第9期320-325,共6页Pengcheng Su Shizheng Chen Zhihong Yang Ningning Zhong Chenzi Jiang Wanbin Li 
financially supported by National Natural Science Foundation of China(No.22178143);Guangdong Basic and Applied Basic Research Foundation(Nos.2021A1515110365 and2020B1515120036);Natural Science Foundation of Anhui Higher Education Institutions(No.2023AH050168);Innovation and Entrepreneurship Training Program for China College Students(No.202310878049);Director Foundation of Anhui Province Engineering Laboratory of Advanced Building Materials(No.JZCL2305ZR);Ph.D.Startup Foundation of Anhui Jianzhu University(No.2023QDZ34)。
Hypercrosslinked polymers(HCPs)with large surface areas,high intrinsic porosities and low production costs may be available platforms for iodine capture.However,the lack of iodine-philicity binding sites limits their ...
关键词:Porous polymers Postsynthetic amination Hypercrosslinked polymers Vapor-phase grafting Iodine capture 
Enhanced conductivity and stability of Prussian blue cathodes in sodium-ion batteries by surface vapor-phase molecular selfassembly被引量:2
《Nano Research》2024年第5期4221-4230,共10页Tao Yuan Xiaopan Fu Yuan Wang Mingjie Li Shuixin Xia Yuepeng Pang Shiyou Zheng 
support of the National Natural Science Foundation of China(Nos.22379096,52271222,51971146,51971147,52171218,52371230);support of Shanghai Outstanding Academic Leaders Plan,the Innovation Program of Shanghai Municipal Education Commission(No.2019-01-07-00-07-E00015);Shanghai Pujiang Program(No.21PJ1411100);Shanghai Rising-Star Program(Nos.20QA1407100,21QA1406500);the Shanghai Science and Technology Commission(Nos.21010503100,20ZR1438400,22ZR1443900).
With many merits such as facile synthesis,economy,and relatively high theoretical capacity,Prussian blue analogs(PBAs)are considered promising cathode materials for sodium-ion batteries(SIBs).However,their practical a...
关键词:sodium-ion battery CATHODE Prussian blue analogs surface modification vapor-phase molecular self-assembly 
Rational construction of multiple hollow silicalite-1 zeolite with enhanced quasi acidity for robust vapor-phase Beckmann rearrangement被引量:2
《Nano Research》2023年第5期7958-7966,共9页Peng Zhang Xianfeng Yi Changjiu Xia Xinxin Peng Shuai Zhang Chengxiang Li Anmin Zheng Xiaoxin Zhang Yibin Luo Lifeng Cui Fuhong Yu Xingtian Shu 
the National Key Basic Research Development Plan“973”Project(No.2006CB202508);the National Key R&D Program of China(No.2021YFA1502600);State Key Laboratory of Catalytic Materials and Reaction Engineering(RIPP,SINOPEC)(No.33600000-20-ZC0607-0024);the SINOPEC Project(Nos.411058 and 413025);the National Natural Science Foundation(Nos.21808244,22178347,and 22072182).
Developing efficient and stable zeolites for vapor-phase Beckmann rearrangement of cyclohexanone oxime is still a great challenge to realizeε-caprolactam(CPL)green production.In this work,the hierarchical porous sili...
关键词:hollow silicalite-1 H-bonded silanols quasi acidity vapor-phase Beckmann rearrangement 
Vapor-Phase Precise-Synthesis of 2D Inorganic Materials for Optoelectronics
《Chinese Journal of Chemistry》2023年第7期825-834,共10页Xing Zhou Fuwei Zhuge Han Wang Tianyou Zhai 
supported by the National Natural Science Foundation of China(Grant Nos.21825103,52172144,and U21A2069);the Ministry of Science and Technology of China(2021YFA1200500).
Comprehensive Summary 2D materials have attracted intensive attention due to their unique electrical and optical properties associated with their strictly defined low dimensionalities.They provide a wide range of basi...
关键词:2D materials HETEROSTRUCTURES Chemical vapor deposition Photoelectric performances Nanostructures photodetectors 
Scalable fabrication of Bi_(2)O_(2)Se polycrystalline thin film for near-infrared optoelectronic devices applications
《Chinese Physics B》2021年第10期470-475,共6页Bin Liu Hong Zhou 
supported by the Hunan Provincial Natural Science Foundation of China(Grant No.2019JJ40032)。
We present a controlled,stepwise formation of layered semiconductor Bi_(2)O_(2)Se thin films prepared via the vapour process by annealing topological insulator Bi_(2)Se3 thin films in low oxygen atmosphere for differe...
关键词:thin films Bi_(2)Se_(3) vapor-phase deposition PHOTODETECTOR Bi_(2)O_(2)Se 
Recovery of free volume in PIM-1 membranes through alcohol vapor treatment被引量:1
《Frontiers of Chemical Science and Engineering》2021年第4期872-881,共10页Faiz Almansour Monica Alberto Rupesh S.Bhavsar Xiaolei Fan Peter M.Budd Patricia Gorgojo 
Faiz Almansour is grateful to the Department of Research&Development,Saudi Aramco for funding and supporting his Ph.D.studies.M.Alberto is grateful to EPSRC for funding under the research grant number EP/S032258/1;R.Bhavsar to EPSRC under grant number EP/M001342/1.
Physical aging is currently a major obstacle for the commercialization of PIM-1 membranes for gas separation applications.A well-known approach to reversing physical aging effects of PIM-1 membranes at laboratory scal...
关键词:polymer of intrinsic microporosity(PIM) PIM-1 physical aging gas separation vapor-phase regeneration 
Vapor-phase decomposition of dimethyl methylphosphonate (DMMP),a sarin surrogate,in presence of metal oxides
《Defence Technology(防务技术)》2021年第4期1095-1114,共20页Shomik Mukhopadhyay Mirko Schoenitz Edward L.Dreizin 
This work was supported by the US Defense Threat Reduction Agency,DTRA;Grant HDTRA1-19-1-0023.
Chemical warfare agents(CWA)are stockpiled in large quantities across the globe.Agents stored in inaccessible facilities need to be destroyed rapidly without dispersing the compounds to surrounding areas.Metal-based e...
关键词:Chemical weapon agents Prompt defeat Metal combustion Heterogeneous reactions 
Solvent-Less Vapor-Phase Fabrication of Membranes for Sustainable Separation Processes
《Engineering》2020年第12期1432-1442,共11页Junjie Zhao Karen K.Gleason 
Zhejiang University,the research grant from the State Key Laboratory of Chemical Engineering(SKL-ChE-19T04);the funding support from the Institute of Zhejiang University-Quzhou(IZQ2019-KJ-011);Junjie Zhao also acknowledges the funding from the National Natural Science Foundation of China(21908194 and 21938011).
Sustainable processes for purifying water,capturing carbon,producing biofuels,operating fuel cells,and performing energy-efficient industrial separations will require next-generation membranes.Solvent-less fabrication...
关键词:Membrane separation Chemical vapor deposition Atomic layer deposition Molecular layer deposition Thin films Metal-organic frameworks POLYMERS Advanced manufacturing 
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