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This work was financially supported by the National Natural Science Foundation of China(Nos.52072371 and 51871209);Key Technologies Research and Development Program of Anhui Province(No.202004a06020056);Special Foundation of President of HFIPS(No.YZJJ202102),HFIPS Director’s Fund(Nos.GGZX GTCX-2023-07 and YZJJ-GGZX-2022-01);HFIPS Director’s Fund(No.2023YZGH05).
Utilization and storage are the two main themes of green hydrogen.In hydrogen-involved system,development of highly active catalysts to achieve catalytic hydrogenation under mild conditions is a prerequisite for coupl...
the National Natural Science Foundation of China(NSFC)(No.22275126);the Natural Science Foundation of Sichuan Province(No.2023NSFSC0634);the Open Project of Key State Laboratory for Supramolecular Structures and Materials of Jilin University(No.SKLSSM 2024036);gratitude for NSFC(No.32000934)and the Natural Science Foundation of Sichuan Province(No.24NSFSC6433);for NSFC(No.22305162);the discussion on experimental data.For TEM,we thank College of Chemistry of Sichuan University(Dr.Feng Yang).
Little is known about the synthesis of colloidal ternary semiconductor magic-size clusters(MSCs)and quantum dots(QDs)in an aqueous environment.We report here the first synthesis of aqueous-phase CdSeS MSC-380(displayi...
supported by the National Natural Science Foundation of China(52061135103,51873236,52203287);Fundamental Research Funds for the Central Universities,Sun Yat-sen University(No.23yxqntd002).
Chiral covalent organic frameworks(COFs)have shown promising applications in asymmetric catalysis,enantiomer separation and chiral recognition due to their tunable structures and permanent porosity.Currently,synthesis...
supported by the National Natural Science Foundation of China(No.22008041);the Natural Science Foun-dation of Guangxi Province,China(Nos.2019GXNSFDA245020 and 2020GXNSFGA297001).
Water-assisted proton hopping(WAPH)plays an important role in the aqueous-phase hydrogenation of levulinic acid(LA)toγ-valerolactone(GVL).In this study,based on a strategy of spontaneously polarized ceramic(SPCE)-rei...
supported by the National Natural Science Foundation of China(Nos.21976034,42077193,92044301,and21906024);the Shanghai Municipal Health Commission Science and Research Fund(No.202040185);the Shanghai Pudong New District Bureau of Ecology and Environment Research Project(No.PDHJ20210008);the Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Great Bay Area(No.2021B1212050024)。
The reaction of carbonyl-to-imine/hemiaminal conversion in the atmospheric aqueous phase is a critical pathway to produce the light-absorbing N-containing secondary organic compounds(SOC).The formation mechanism of th...
supported by the National Natural Science Foundation of China(Nos.91844301 and 42005087);the support from State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex,Shanghai Academy of Environment Sciences(No.CX2020080581)。
Aerosol liquid water content(ALWC)plays an important role in secondary aerosol formation.In this study,a whole year field campaign was conducted at Shanxi in north Zhejiang Province during 2021.ALWC estimated by ISORR...
supported by the National Natural Science Foundation of China(Nos.22171002 and 21603001);the Wanjiang Scholar Program,and the Natural Science Foundation of Anhui Province(No.2108085MB54).
1.Introduction Metal ions have played a vital role in various living systems and in-dustrial applications for a long time[1].Among them,Fe3+is a basic component of hemoglobin,and undertakes the responsibility of biolo...
Project supported by National Natural Science Foundation of China(21868026,22006079);the National First-class Discipline Construction Project;the Project of Ningxia Key R&D Plan(2020BEB04009)。
Hydrodeoxygenation(HDO)of renewable lignin-derived biomass in aqueous-phase to produce high value-added products is of great significance.However,developing new catalysts with high activity and excellent stability in ...
Solid-aqueous interfaces and phenomena occurring at those interfaces are ubiquitously found in a plethora of chemical systems.When it comes to heterogeneous catalysis,however,our understanding of chemical transformati...
K.Y.thanks the National Natural Science Foundation of China(No.21773162);the Fundamental Research Funds for the Central Universities,the Applied Basic Research Programs of Science and Technology Department of Sichuan Province(No.2020YJ0326);the State Key Laboratory of Polymer Materials Engineering of Sichuan University(No.sklpme2020-2-09);the Open Project of Key State Laboratory for Supramolecular Structures and Materials of Jilin University(No.SKLSSM 2021030);the National Major Scientific and Technological Special Project for“Significant New Drugs Development”(No.2019ZX09201005-005-002);M.Z.is grateful to the National Natural Science Foundation of China(No.22002099);China Postdoctoral Science Foundation(No.2020T130441);Sichuan University postdoctoral interdisciplinary Innovation Fund,and the Open Project of Key State Laboratory for Supramolecular Structures and Materials of Jilin University(No.SKLSSM 2021032).
The formation pathway of aqueous-phase colloidal semiconductor magic-size clusters(MSCs)remains unrevealed.In the present work,we demonstrate,for the first time,a precursor compound(PC)-enabled formation pathway of aq...