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Enhancing anion conductivity in a highly alkali-stable eta topologic Cu(Ⅰ)framework via strong electrostatic repulsion
《Science China Chemistry》2025年第3期980-986,共7页Xiao-Lu Wang Shaohui Guo Chao Suo Fu-Qiang Zhang Jun-Hao Wang Wenjing Wang Daqiang Yuan Linfeng Liang Xian-Ming Zhang 
supported by the Fundamental Research Program of Shanxi Province (202403021212028);the National Natural Science Foundation of China (22001154);the Central Government Funding for Talent Promotion (231545023);the Youth Fund from the Department of Science and Technology of Shanxi Province (201901D211148);the Science and Technology Innovation Planning Project in Universities and Colleges of Shanxi Province (2019L0063)。
Metal-organic frameworks(MOFs)based on anion exchange membranes(AEMs)have garnered considerable interest,particularly for their potential to enhance ion conductivity by pre-introducing anions into MOFs.This approach i...
关键词：metal-organic framework crystal engineering ionic conduction 
A highly reduced Mo_(74) polyoxometalate featuring high proton conductivity accessed by building block strategy被引量：1
《Science China Chemistry》2024年第3期862-868,共7页Shi-Yi Liu Xue-Xin Li Wei-Chao Chen Kui-Zhan Shao Xin-Long Wang Chao Qin Zhong-Min Su 
supported by the Natural Science Foundation of Jilin Province-Free Exploration General Project(YDZJ202201ZYTS331);the National Natural Science Foundation of China(21801038);the Science and Technology Research Foundation of Jilin Educational Committee(JJKH20221158KJ);the Fundamental Research Funds for the Central Universities(2412022ZD002,2412022ZD009)。
Highly reduced polyoxometalates(POMs) are predicted to be used as rather high energy density materials;however,it still suffers from the limited cluster species and reduction ratio.Here we demonstrate that it is possi...
关键词：POLYOXOMETALATE building block MOLYBDENUM highly reduced state proton conduction 
A silylene-stabilized distannavinylidene with a highly labile substituent
《Science China Chemistry》2023年第12期3555-3561,共7页Zihao Qiao Ming Chen Zhenbo Mo 
supported by the National Natural Science Foundation of China(22071124,22371130,22221002);the Frontiers Science Center for New Organic Matter at Nankai University(C029215001);the Fundamental Research Funds for the Central Universities(63206007);the Nankai University and Young Elite Scientists Sponsorship Program by Tianjin。
Vinylidene and its heavier analogues are fundamentally important in synthetic chemistry,but their stabilization and structural characterization remains extremely challenging.Herein we describe that the reduction of an...
关键词：distannavinylidene SILYLENES stannacycles distannyne CARBORANES 
Understanding the sluggish and highly variable transport kinetics of lithium ions in LiFePO_4被引量：1
《Science China Chemistry》2023年第11期3297-3306,共10页Youcheng Hu Xiaoxiao Wang Peng Li Junxiang Chen Shengli Chen 
financially supported by the National Natural Science Foundation of China(22272122,21832004 and 21673163)。
LiFePO_(4),one of the mainstream cathode materials of current EV batteries,exhibits experimental diffusion coefficients(D_(c))of Li^(+)which are not only several orders of magnitude lower than those predicted by the i...
关键词：lithium iron phosphate diffusion coefficient machine-learning potential kinetic Monte Carlo simulations 
Highly stable Eu-coordination polymer exhibiting the highest quantum yield
《Science China Chemistry》2023年第5期1400-1405,共6页Ming-Yu Ye Ming-Xuan Zhang Qiao-Fei Xu Han Xu La-Sheng Long Lan-Sun Zheng 
supported by the National Natural Science Foundation of China(92161203,21721001,22022108)。
Lanthanide luminescent materials with high quantum yield and thermal stability are of key importance for their practical application.Here we report crystal structures and luminescent properties of[Eu(pfbz)_(2)(phen)Cl...
关键词：LANTHANIDE coordination polymers LUMINESCENCE LED materials 
Metal-free multicomponent polymerization of activated diyne,electrophilic styrene and isocyanide towards highly substituted and functional poly(cyclopentadiene)
《Science China Chemistry》2023年第3期863-869,共7页Xinyue Liu Xueqin Yang Xin Li Jianwei Sun Benzhao He Jacky W.Y.Lam Ben Zhong Tang 
supported by the National Natural Science Foundation of China(21788102,22101028);the Research Grants Council of Hong Kong(16304819,16305320,C6014-20W);the Innovation and Technology Commission(ITC-CNERC14SC01);the Natural Science Foundation of Guangdong Province(2019B121205002);Shenzhen Key laboratory of Functional Aggregate Materials(ZDSYS20212021222400001);the Nissan Chemical Industries,Ltd.
The development of a facile and efficient polymerization to prepare cyclopentadiene-containing polymers is of vital importance and highly desired. In this work, a metal-free multicomponent polymerization of activated ...
关键词：multicomponent polymerization activated alkynes highly substituted poly(cyclopentadiene) 
Facet-selective growth of MOF-on-MOF heterostructures enables etching-free synthesis of highly-open Co/N-doped carbon nanoframes for efficient catalysis
《Science China Chemistry》2022年第12期2450-2461,共12页Yaohui Wu Liyu Chen Xianfeng Yang Yingwei Li Kui Shen 
supported by Guangdong Natural Science Funds for Distinguished Young Scholar(2018B030306050);the National Natural Science Foundation of China(22138003,21825802);the Natural Science Foundation of Guangdong Province(2017A030312005).
Highly-open nanoframe structures consisting of interconnected and exposed ridges are highly desirable for achieving efficient catalysis,but preparing them by a facile etching-free methodology is still a very daunting ...
关键词：metal-organic frameworks etching-free synthesis highly-open nanoframes pyrolysis efficient catalysis 
The “twinkling star” materials: highly superior molecular switches for bioimaging
《Science China Chemistry》2019年第6期657-658,共2页Qi Zou 
Artificial molecular switches have been the robust tools for diverse fields of modern science and technology, including molecular machines, smart materials, and bioimaging [1]. The development of new concepts to enabl...
关键词：MOLECULAR development STATES 
Highly enantioselective cyclopropanation of trisubstituted olefins被引量：2
《Science China Chemistry》2018年第5期526-530,共5页Jun Li Long Zheng Hao Chen Lijia Wang Xiu-Li Sun Jun Zhu Yong Tang 
supported by the National Natural Science Foundation of China(21432011,21772224);Key Research Program of Frontier Sciences of Chinese Academy of Sciences(QYZDY-SSWSLH016);the Strategic Priority Research Program of the Chinese Academy of Sciences(XDB20000000);the Youth Innovation Promotion Association CAS(2017301);the National Basic Research Program of China(2015CB856600)
A highly efficient asymmetric cyclopropanation of trisubstituted olefins with methyl diazoacetate has been developed in terms of an elaborate modified chiral bisoxazoline/copper complex as a catalyst. A broad scope of...
关键词：cyclopropanation enantioselective bisoxazoline copper diazoacetate 
Direct and highly selective conversion of CO_2 into gasoline fuels over a bifunctional catalyst
《Science China Chemistry》2017年第9期1145-1146,共2页Mingyuan He 
CO2 is an economical, nontoxic, renewable and abundant car-bon source. The chemical utilization of CO2 into value-addedproducts is very attractive because it can not only alleviatethe global warming caused by increasi...
关键词：中国科学 化学英文版 
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