supported by the National Natural Science Foundation of China(grant nos.22071146 and 21931005);the Shanghai Science and Technology Committee(grant no.23XD1421800);the Shanghai Shuguang Program(grant no.21SG12);the Shanghai Municipal Science and Technology Major Project.
The mass production of urea,the most widely used agricultural fertilizer,usually relies on energy-and carbon-intensive processes.The light-driven synthesis path has great potential for more sustainable techniques to p...
supported by the National Natural Science Foundation of China(grant no.22278056);the Liaoning Provincial Natural Science Foundation(grant no.2023-MS-105);the Liaoning Revitalization Talents Program(grant no.XLYC3008032);the Fundamental Research Funds for the Central Universities(grant no.DUT22LAB602).
Selective photocatalytic reduction of carbon dioxide(CO_(2))to specific C2 and C1 products is highly desirable.The present work is a computational screening of the photocatalytic performance of a series of Cu-M dual-m...
supported by National Key R&D Program of China(grant no.2022YFA1502902);the National Natural Science Foundation of China(grant nos.22371208,22271218,22071182,and 21931007);the Science&Technology Development Fund of Tianjin Education Commission for Higher Education(grant no.2018KJ129).
Photocatalytic CO_(2)reduction into chemical fuels is a promising route for alleviating the energy crisis and environmental issues.However,reported catalysts still exhibit low catalytic efficiencies,which hinders the ...
the funding from the National Natural Science Foundation of China(grant nos.22072065,22178162,and 22222806);the Distinguished Youth Foundation of Jiangsu Province(grant no.BK20220053);the Six Talent Peaks Project in Jiangsu Province(grant no.JNHB-035);Agency for Science,Technology and Research(A*STAR)through Low Carbon Energy Research Finding Initiative(grant nos.LCERFI01-0033 and U2102d2006).
Finely adjusting the local environment of Cu single atom(SA)is crucial but challenging for the fabrication of electrocatalysts for the CO_(2)reduction reaction(CO_(2)RR)to produce clean energy methane(CH_(4)).Herein,p...
supported by the National Key Research and Development Program of China(grant nos.2023YFA1507904 and 2021YFA1501500);National Natural Science Foundation of China(grant nos.U22A20436,22071245,22220102005,and 22033008);Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China(grant no.2021ZZ103);Talent Plan of Shanghai Branch,Chinese Academy of Sciences(grant no.CASSHB-QNPD-2023-020);supported by the Open Science Promotion Plan 2023 of China Science and technology Cloud.The authors thank the Taiwan beamline BL-12B2 at SPring-8(Japan)and the beamline TPS 44A of the National Synchrotron Radiation Research Center for EXAFS measurements.
Developing nonmetallic active sites-based catalysts for efficient electrocatalytic CO_(2)reduction reaction(CO_(2)RR)remains challenging.Active N-heterocyclic carbenes(NHCs)as typical nonmetal catalysts have shown hig...
supported by National Natural Science Foundation of China(grant nos.21821005,21931012,21820102002,22293043,52272097,and 52202354);the Beijing Natural Science Foundation(grant no.2242019);the DNL Cooperation Fund,Chinese Academy of Sciences(CAS)(grant no.DNL202020).
The ultimate goal of photocatalytic CO_(2)reduction is to efficiently convert atmospheric CO_(2)into value-added products by designing hierarchical photocatalysts that combine effective harvesting and accelerate activ...
supported by the National Key R&D Program of China(grant nos.2022YFA1502903 and 2021YFA1501502);the Strategic Priority Research Program of the Chinese Academy of Sciences(CAS;grant nos.XDB0450000 and XDB36000000);the National Natural Science Foundation of China(grant nos.92163105,T2122004,U2032212,and 22275179);Anhui Provincial Key Research and Development Program(grant no.2022a05020054);the China Postdoctoral Science Foundation(CPSF;grant nos.2023TQ0341 and 2023M743369);the Youth Innovation Promotion Association of CAS(grant no.Y2021123);the Fundamental Research Funds for the Central Universities(grant nos.WK2060000039 and WK2060000068);the Postdoctoral Fellowship Program of CPSF(grant no.GZB20230706).
In nature,green leaves accomplish photosynthesis via chloroplasts,where the Mg-N4-centered chlorophyll and enzymes undertake light absorption and catalytic reaction,involving CO_(2)fixation,with the resultant six-carb...
Introduction to the Special Issue on CO_(2)Capture and Conversion Concerns over climate change and its catastrophic consequences have spurred an intense global effort to investigate technologies for reducing atmospher...
Christopher Jones Prof.Jones received his B.S.E.from the University of Michigan,USA,in 1995,followed by his M.S.(1997)and Ph.D.(1999)in Chemical Engineering from the California Institute of Technology(CalTech),USA,wit...
financially supported by the Division of Chemical Sciences,Geosciences,&Biosciences,Office of Basic Energy Sciences(contract number DESC0012704)of the U.S.Department of Energy.
The growing global climate crisis linked to rising atmospheric CO_(2)levels calls for urgent and innovative solutions.Fixing CO_(2)as valuable solid carbon products,such as carbon nanofibers or nanotubes(CNFs or CNTs)...