国家自然科学基金(20923006)

作品数:12被引量:13H指数:2
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相关作者:贡卫涛宁桂玲高岩张敏孙立成更多>>
相关机构:大连理工大学瑞典皇家工学院吉林大学第一医院更多>>
相关期刊:《分子科学学报》《Journal of Energy Chemistry》《Chinese Journal of Catalysis》《中国科学:化学》更多>>
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Insights into electrolyte effects on photoactivities of dye-sensitized photoelectrochemical cells for water splitting
《Journal of Energy Chemistry》2017年第3期476-480,共5页Xin Ding Linlin Zhang Yan Gao 
supported by the National Basic Research Program of China(973 program,2014CB23940);the National Natural Science Foundation of China(20923006,21120102036,91233201 and 21573033);the Natural Science Foundation of Shandong Province(ZR2016BB14);the Postdoctoral innovation Foundation of Shandong Province(201602039);the Fundamental Research Funds for the Central Universities(DUT13RC(3)103,DUT15LK08);the Basic Research Project of Key Laboratory of Liaoning(LZ2015015);the State Key Laboratory of Fine Chemicals(KF1513)
Dye-sensitized photoelectrochemical cell(DS-PEC) is an especially attractive method to generate hydrogen via visible light driven water splitting. Electrolyte, an essential component of DS-PEC, plays a great role in...
关键词:Water splitting Molecular device PHOTOANODE ELECTROLYTE DS-PEC 
Influences of the adsorption state of catalyst on the performance of DS-PEC for visible light driven water splitting
《Journal of Energy Chemistry》2017年第1期163-167,共5页Linlin Zhang Yan Gao Xin Ding 
supported by the National Basic Research Program of China(973 Program)(2014CB23940);the National Natural Science Foundation of China(20923006,21120102036,91233201 and 21573033);the Fundamental Research Funds for the Central Universities(grant number DUT13RC(3)103,DUT15LK08);the China Postdoctoral Foundation 2015M582157;the State Key Laboratory of Fine Chemicals(KF1513);the Basic Research Project of Key Laboratory of Liaoning(LZ2015015)
Adsorption state of catalyst on photoanode is an important factor on influencing the performance of dye-sensitized photoelectrochemical cells (DS-PECs) for water splitting. Photoanode TiO2(1 + 2) was assembled with Ru...
关键词:Water oxidation PHOTOELECTROCHEMICAL PHOTOANODE DS-PEC 
新型菲并二氧化噻二唑类染料的合成及性能
《分子科学学报》2016年第4期309-314,共6页张新 刘杜 江华 吴杰 
国家自然科学基金委专项基金资助项目(20923006)
设计合成了4种以菲并二氧化噻二唑结构为电子受体、三苯胺或N,N-二(4-正丁基苯基)苯胺结构为电子给体的D-A-D型纯有机功能染料5a,5b,6a和6b.利用紫外-可见吸收光谱、荧光发射光谱、循环伏安曲线及理论计算对该染料的光学、电化学性质进...
关键词:染料 吸收 菲并二氧化噻二唑 三苯胺 
溴的吸电子效应对Ru-bda(H2bda=2,2′-联吡啶-6,6′-二羧基)型催化剂催化水氧化的性能影响(英文)被引量:2
《催化学报》2015年第10期1742-1749,共8页刘昭 高岩 于泽 张敏 刘建辉 
supported by the National Basic Research Program of China(973 program)(2014CB239402);the National Natural Science Foundation of China(20923006,21120102036,21106015,91233201);the Fundamental Research Funds for the Central Universities(DUT13RC(3)103,DUT15LK08)~~
太阳能高效转化和利用是实现能源结构调整、节能减排、保障社会健康发展的重要途径.光解水制氢是实现太阳能转化成化学能,解决能源需求和环境污染一个理想方法,其中水氧化反应是制约太阳能转化的关键.近几十年来,科学家们一直致力于开...
关键词:水氧化 Ru-bda型催化剂 溴取代 吸电子效应 动力学研究 
基于分子催化剂光驱动水氧化器件的研究进展被引量:1
《中国科学:化学》2014年第4期625-630,共6页高岩 段丽娜 张敏 孙立成 
国家自然科学基金(20923006,21003017,21120102036,21106015和91233201)的资助
光解水制氢是人们解决未来能源危机的一种重要构想,构建高效的光电化学池是实现这一构想的重要途径,而光驱动水氧化的顺利进行是实现这一过程的关键.本文总结了近年来基于分子催化剂及染料敏化的光驱动水氧化分子器件的研究和进展,介绍...
关键词:光解水 光电化学池 水氧化 分子器件 
Palladium-Catalyzed Desulfitative Cross-Coupling of Sodium Arylsulfinates with Aryl Bromides and Chlorides: An Alternative Convenient Synthesis of Biaryls被引量:1
《Chinese Journal of Chemistry》2013年第10期1269-1273,共5页Chao Zhou Yarning Li Yang Lu Rong Zhang Kun Jin Xinmei Fu Chunying Duan 
Acknowledgement This work was supported by the National Natural Science Foundation of China (Nos. 21176039, 20876021 and 20923006).
An alternative method for synthesis of biaryls has been developed through the Pd catalyzed desulfitative coupling reaction of sodium arylsulfinates with aryl bromides and chlorides. The procedure tolerates a variety o...
关键词:CROSS-COUPLING desulfination aryl bromides aryl chlorides PALLADIUM 
单核钌催化剂化学催化和光催化水氧化反应(英文)被引量:1
《催化学报》2013年第8期1489-1495,共7页姜毅 李斐 黄芳 张彪彪 孙立成 
supported by the National Basic Research Program of China (973 Program,2009CB220009);the National Natural Science Foundation of China (21106015,21120102036,and 20923006);the Research Fund for the Doctoral Program of Higher Education of China (20110041120005);the Swedish Energy Agency and K&A Wallenberg Foundation~~
合成了一系列含有不同对位取代基团的吡啶轴向配体的单核钌化合物Ru(bda)(pic)2(H2bda = 2,2'-联吡啶-6,6'-二羧酸; pic =对甲基吡啶), 对化合物的结构进行了核磁、质谱和X射线单晶衍射表征, 并在中性和酸性条件下研究了这些化合物的电...
关键词:分解水 水氧化 钌配合物 吸电子效应 光催化 
Synthesis of a water-soluble macromolecular light stabilizer containing hindered amine structures被引量:5
《Chinese Chemical Letters》2013年第2期153-155,共3页Wei Ma Mei Meng Xue Jiang Bing-Tao Tang Shu-Fen Zhang 
the financial support of the National Natural Science Foundation of China(Nos.20806013, 20923006);the National Key Technology R&D Program(No. 2011BAE07B08)
Received 26 September 2012 Received in revised form 18 December 20 Accepted 1 January 2013 Available online 4 February 2013
关键词:Water-soluble macromolecular lightstabilizerHindered amineLightfastness of reactive dyesFinishing 
Synthesis and Characterization of New Thienopyrazine-cored Dendrimer for Non-Doped Organic Red Light-Emitting Diodes
《Chinese Journal of Chemistry》2011年第12期2655-2658,共4页李青 李久艳 段永恒 高占先 刘迪 
Project supported by the National Natural Science Foundation of China (Nos. 20704002, 20923006, 21072026), the Ministry of Education for the New Century Excellent Talents in University (No. NCET-08-0074), and the Fundamental Research Funds for the Central Universities (No. DUT 10LK 16).
A new thieno-[3,4-b]-pyrazine-cored dendrimer with polyphenyls dendrons (D2TP) was designed and synthesized for application as red emitter in non-doped organic light-emitting diodes (OLEDs). The bulky dendritic ar...
关键词:thienopyrazine DENDRIMER light-emitting diodes red electroluminescence 
2,4,6-三苯基吡喃盐与三烷基(芳基)膦的新型共轭加成反应
《有机化学》2011年第10期1707-1709,共3页徐涛 贡卫涛 叶俊伟 宁桂玲 林源 
国家自然科学基金(No.20772014);中央高校基本科研业务费专项资金(No.1000-893116);国家自然科学基金委专项基金(No.20923006)资助项目
研究发现,2,4,6-三苯基吡喃盐与三烷基(芳基)膦化合物PR3(R=Me,Et,Ph)可以发生两分子的共轭加成反应,生成结构新颖的开环产物季鏻盐1.通过1H NMR,13C NMR,31P NMR,质谱和元素分析表征,确定了反应产物的最终结构.
关键词:三烷基(芳基)膦 共轭加成 吡喃盐 季鏻盐 
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