ELECTRON-DEFICIENT

作品数：35被引量：63H指数：4
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相关领域：理学更多>>
相关作者：王刚伟杨尚东张恒颜朝国侯秀峰更多>>
相关机构：武汉大学兰州大学北京大学复旦大学更多>>
相关期刊：《Green Energy & Environment》《Nano-Micro Letters》《Science China Chemistry》《Journal of Energy Chemistry》更多>>
相关基金：国家自然科学基金中国博士后科学基金俄罗斯基础研究基金国家重点基础研究发展计划更多>>
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Electrochemical Carboarylation of Activated Alkenes with CO_(2)and Electron-deficient Aryl Bromides
《Chinese Journal of Chemistry》2024年第24期3367-3372,共6页Zhaoliang Yang Chunlei Liu Cheng Zhong Jianye Zhang Shengzhang Liu mingming Yu yangyang Li Hong Yi Aiwen Lei 
supported by the National Key R&D Program of China(2022YFA1505100,2021YFA1500104);National Natural Science Foundation of China(22031008,22201222);Science Foundation of Wuhan(2023020201020266,2020010601012192);Jiangxi Normal University Doctoral Research Initiation Fund Project(12017081,12022796).
The simultaneous construction of two vicinal C—C bonds in a molecule remains a significant challenge.In this work,we disclose an electroreductive carboarylation of activated alkenes under mild,transition metal-free c...
关键词：Electroreductive Difunctionalization Carboarylation Activated alkenes CO_(2) Aryl bromides 
Tailoring Electrode–Electrolyte Interface Using an Electron-Deficient Borate-Based Additive in MgTFSI_(2)-MgCl_(2)/DME Electrolyte for Rechargeable Magnesium Batteries
《Energy & Environmental Materials》2024年第6期167-175,共9页Haiyan Fan Xinxin Zhang Jianhua Xiao Wenjie Chen Qiyuan Lin Zi Shyun Ng Yitao Lin Yi Su Ludi Pan Yipeng Su Shuaiyang Ren Haowen Liu Xuanzhang Li Yuegang Zhang 
supported by the National Natural Science Foundation of China(22150710516,U1832218).
Rechargeable magnesium metal batteries need an electrolyte that forms a stable and ionically conductive solid electrolyte interphase(SEI)on the anodes.Here,we used molecular dynamic simulation,density functional theor...
关键词：electrolyte additives interfacial chemistry magnesium metal batteries solvation structure 
Promoting electroreduction of nitrite to ammonia over electron-deficient Pd modulated by rectifying Schottky contacts
《Journal of Energy Chemistry》2024年第11期524-530,共7页Shaobo Zhang Yabo Guo Lu-Hua Zhang Zhihao Feng Bo Zhang Yaheng Wang Fengshou Yu 
Electrochemical nitrite reduction reaction(NO_(2)^(-)RR) is a potential sustainable route for regulating the nitrogen cycle and ambient ammonia(NH_(3)) synthesis.However,it remains a challenge to precisely regulate th...
关键词：ELECTROCATALYTIC Nitrite reduction reaction Electronic structure AMMONIA 
A new class of crystalline X-ray induced photochromic materials assembled from anion-directed folding of a flexible cation
《Chinese Chemical Letters》2024年第8期554-557,共4页Hong-Jin Liao Zhu Zhuo Qing Li Yoshihito Shiota Jonathan P.Hill Katsuhiko Ariga Zi-Xiu Lu Lu-Yao Liu Zi-Ang Nan Wei Wang You-Gui Huang 
supported by National Natural Science Foundation of China(No.92261109);Natural Science Foundation of Fujian Province(No.2020J05080);Project Funded by China Postdoctoral Science Foundation(No.2023M733496);Natural Science Foundation of Xiamen(No.3502Z20206080);Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China(No.2021ZR110);Recruitment Program of Global Youth Experts,Youth Innovation Promotion Association CAS(No.2021302).
Electron-deficient viologens are widely used as ligands or structure-directing agents(SDAs)to synthesize crystalline X-ray induced photochromic materials.Here,a new rational strategy of anion-directed fold-ing a flexi...
关键词：Supramolecular Photochromic X-ray induced Anion-directed folding Electron-deficient viologens 
Electron-deficient ZnO induced by heterointerface engineering as the dominant active component to boost CO_(2)-to-formate conversion
《Carbon Energy》2024年第5期127-136,共10页Qing Qin Zijian Li Yingzheng Zhang Haeseong Jang Li Zhai Liqiang Hou Xiaoqian Wei Zhe Wang Min Gyu Kim Shangguo Liu Xien Liu 
National Natural Science Foundation of China,Grant/Award Number:22102079;Taishan Scholar Program of Shandong Province,China,Grant/Award Number:tsqn202211162;Natural Science Foundation of Shandong Province of China,Grant/Award Numbers:ZR2021YQ10,ZR2022QB163。
Electrocatalytic CO_(2)-to-formate conversion is considered an economically viable process.In general,Zn-based nanomaterials are well-known to be highly efficient electrocatalysts for the conversion of CO_(2) to CO,bu...
关键词：charge redistribution CO_(2)reduction reaction ELECTROCATALYST heterointerfaces SELECTIVITY 
On-Surface Synthesis of Electron-Deficient Bisanthene Tetraimide
《CCS Chemistry》2024年第3期672-681,共10页Ye Liu Liangliang Chen Hailong Li Xi-Sha Zhang Qigang Zhong Zhengming Hao Minghui Wu Yan-Ying Huang Lina Wang Minchong Sheng Miao Xie Haiming Zhang Deqing Zhang Lifeng Chi 
support from the National Natural Science Foundation of China(grant nos.22161132026,21790053,51821002,and 21602225);the Suzhou Key Laboratory of Surface and Interface Intelligent Matter(grant no.SZS2022011);the Collaborative Innovation Center of Suzhou Nano Science and Technology;the Priority Academic Program Development of Jiangsu Higher Education Institutions(PAPD);the 111 project.
Imide-based conjugated molecules have emerged as a highly promising class of building blocks for constructing n-type semiconducting materials with lowlying lowest unoccupied molecular orbitals and exceptional stabilit...
关键词：on-surface synthesis ELECTRON-DEFICIENT bisanthene tetraimide DEHYDROCYCLIZATION low lowest unoccupied molecular orbital level 
Regulating the Electron-Deficient Component in A-DA1D-A Typed Small-Molecule Acceptors for High-Performance Organic Solar Cells
《Chinese Journal of Chemistry》2024年第6期623-630,共8页Weifei Wei Ruijie Ma Zhanxiang Chen Tongle Xu Gang Li Zhenghui Luo 
supported by the Shenzhen Science and Technology Program(ZDSYS20210623091813040,RCBS20221008093225021);the National Natural Science Foundation of China(NSFC,No.22309119);G.Li acknowledges the support from Research Grants Council of Hong Kong(Project Nos.15320216,15221320,C5037-18G,RGC Senior Research Fellowship Scheme(SRFS2223-5S01));the Hong Kong Polytechnic University(Sir Sze-yuen Chung Endowed Professorship Fund(8-8480);PolyU Distinguished postdoc Fellowship(1-YW4C,R.Ma),G-SAC5)。
Fine-tuning of the electron-deficient unit in A-DA1D-A typed small-molecule acceptors (SMAs) plays a crucial role in developing efficient SMAs for organic solar cells (OSCs).Here,we developed a SMA based on benzo[4,5]...
关键词：Organic solar cells Small-molecule acceptor Electron-deficient unit Energy conversion efficiency Renewable resources π-πstacking Green chemistry 
An asymmetric non-fused electron-deficient building block for low-cost polymer acceptor in all-polymer solar cells
《Science China Chemistry》2023年第9期2626-2633,共8页Haiqin Xiao Linfeng Yu Zhiliang Zhang Haiyan Liang Yu Shi Xia Guo Maojie Zhang Yongfang Li 
supported by the National Natural Science Foundation of China (51973146);the Shandong Provincial Natural Science Foundation (ZR2022JQ09);the Collaborative Innovation Center of Suzhou Nano Science & Technology。
The development of polymerized fused-ring small molecule acceptors(FRA-PAs) has boosted the performance of all-polymer solar cells(all-PSCs).However,these FRA-PAs suffer from lengthy synthesis steps and high productio...
关键词：non-fused electron-deficient building block low-cost polymer acceptors batch-to-batch reproducibility all-polymer solar cells 
Asymmetric Dearomatization of Electron-Deficient Heteroarenes by a Phosphine-Catalyzed[3+2]Annulation with Vinylcyclopropanes
《CCS Chemistry》2023年第9期2023-2032,共10页Xuan Dai Fuhao Zhang Lei Dai Yixin Lu 
the NRF Investigatorship Award(A-0004067-00-02);the Ministry of Education(MOE)of Singapore(A-0008481-00-00)for generous financial support.
Asymmetric dearomatization reactions of various electron-deficient heteroarenes,including benzofurans,benzothiophenes,and indoles,have been described.Through a phosphine-catalyzed[3+2]annulation with vinylcyclopropane...
关键词：DEAROMATIZATION ENANTIOSELECTIVITY phosphine catalysis electron-deficient heteroarenes VINYLCYCLOPROPANES 
Electrochemical Umpolung Enabled Radical-Radical Cross-Coupling Between Electron-Deficient Methylarenes and Aldehydes被引量：1
《CCS Chemistry》2023年第9期1973-1981,共9页Fei Lian Kun Xu Chengchu Zeng 
the National Natural Science Foundation of China(grant nos.22271009 and 22171015);Beijing Natural Science Foundation(grant no.2222003);Beijing Municipal Education Committee Project(grant nos.KZ202110005003 and KM202110005006).
The electrochemical utilization of electron-deficient methylarenes for radical-radical cross-couplings remains very rare.Enabled by an umpolung strategy,the unprecedented electrochemical cross-coupling of electron-def...
关键词：paired electrolysis ketyl radical UMPOLUNG radical-radical cross-coupling methylarene ALDEHYDE 
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