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作品数：20被引量：13H指数：2
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相关作者：毕锡和廖沛球吴安心更多>>
相关机构：东北师范大学华中师范大学更多>>
相关期刊：《Science China Chemistry》《Chemical Research in Chinese Universities》《Chinese Journal of Polymer Science》《合成化学》更多>>
相关基金：国家自然科学基金美国国家科学基金国家高技术研究发展计划国家教育部博士点基金更多>>
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Tandem asymmetric propargylic amination/carboxylative cyclization reaction to chiral 5-methylidene-2-oxazolidinones using CO_(2) as C1 synthon
《Science China Chemistry》2025年第4期1402-1411,共10页Zheng Zhang Zhi-Hao Zhang Ying Sun Yun-Hao Tang Yi-Zhuo Yang Feng Zhou Jian Zhou 
supported by the National Natural Science Foundation of China(21871090,21725203);the National Key Research and Development Program of China(2020YFA0710200);the Shanghai Science and Technology Innovation Action Plan(20JC1416900);the Innovation Program of Shanghai Municipal Education Commission(2023ZKZD37);the Fundamental Research Funds for the Central Universities.
We report a tandem asymmetric Cu-catalyzed propargylic amination(ACPA)/Ag-catalyzed carboxylative cyclization(SCC)with CO_(2) to 5-methylidene-2-oxazolidinones;even with tetrasubstituted stereocenters.By varying pyrid...
关键词：CO_(2) 2-oxazolidinone tandem sequence propargylic amination carboxylative cyclization 
I_(2)-DMSO-Mediated Multicomponent [2+1+1+1] Annulation Reaction via Ethyl Nitroacetate C-NO_(2), Bond Cleavage as a C1 Synthon: A Route to Multisubstituted β-Pyrrolidinones Derivatives with a Quaternary Center
《Chinese Journal of Chemistry》2024年第17期2029-2034,共6页Zhi-Cheng Yu Xi Shen You Zhou Xiang-Long Chen Li-Sheng Wang Yan-Dong Wu An-Xin Wu 
supported by the National Natural Science Foundation of China(Grant 22171098);supported by Chengdu Guibao Science&Technology Co.,Ltd.and the 111ProjectB17019.
A[2+1+1+1]cyclization reaction has been developed for the synthesis of multisubstituted 6-pyrrolidinones from commercially available aryl methyl ketones,primary amines,and ethyl nitroacetate.In this I_(2)-DMSO-meditat...
关键词：CYCLIZATION Multisubstitutedβ-pyrrolidinones I_(2)-DMSO C1 building blocks Quaternary carbon center Late-stage modification Cracking 
An Isolable Phosphinogermylyne as a Synthon of One-Coordinate GeⅠRadical
《Chinese Journal of Chemistry》2024年第7期736-742,共7页Dongmin Wang Haonan Chen Yuhao He Xiaodan Chen Li Zhang Gengwen Tan 
National Natural Science Foundation of China (Grants:22322112 and 22071164);Fundamental Research Funds for the Central Universities,Sun Yat-sen University (23qnpy35);the Suzhou Science&Technology NOVA Program (Grant:ZXL2022445)for generous financial support;L.Z.thanks Guangxi University of Science and Technology (03190227 and 03190228);the Guangxi Department of Science and Technology (2021GXNSFBA220021)for financial support.
Reduction of chlorogermylene MsFluindtBu-GeCl 1 with potassium graphite(KC8)afforded putative germylyne radical MsFluindtBu-Ge 2 as confirmed by electron paramagnetic resonance(EPR)spectroscopy.However,it slowly decay...
关键词：Phosphinogermylyne GERMANIUM RADICALS Donor-acceptor systems Radical reactions 
Synthesis of 2-Trifluoromethyl-4-aminoquinolines via Heating-Promoted Multi-component Reaction of CF_(3)-Imidoyl Sulfoxonium Ylides and Amines with Difluorocarbene as a C1 Synthon
《Chinese Journal of Chemistry》2023年第23期3205-3210,共6页Guangming Wei Chen Li Haoyuan Wang Zhengkai Chen Xiao-Feng Wu 
financial support from K.C.Wong Education Foundation(GJTD-2020-08).
A thermally-induced multi-component reaction of CF_(3)-substituted imidoyl sulfoxonium ylides(TFISYs),amines and(triphenylphosphonio)difluoroacetate(PDFA)has been developed,allowing a facile access to 2-trifluoromethy...
关键词：CF_(3)-Imidoyl sulfoxonium ylides DIFLUOROCARBENE Multi-component reaction 2-Trifluoromethyl-4-aminoquinolines N-Heterocyclic compounds 
Diastereodivergent formal[4+1]cycloaddition of azoalkenes as one-carbon synthons
《Green Synthesis and Catalysis》2023年第3期258-262,共5页Chun-Yan Guan Tian-Jiao Han Shi-Kun Jia Yuan-Zhao Hua Guang-Jian Mei 
support from the Natural Science Foundation of Henan Province(No.222300420084);the Application Research Plan of Key Scientific Research Projects in Colleges and Universities of Henan Province(No.22A150056)is gratefully acknowledged.
The first diastereodivergent formal[4+1]cycloaddition reactions of azoalkenes with p-quinone methides(pQMs)have been accomplished.The reported reaction occurred via a domino oxa-1,4-addition/1,6-addition process,allow...
关键词：Azoalkene One-carbon synthon Diastereodivergent [4+1]Cycloaddition para-Quinone methides 
Recent advances in chemical fixation of CO_(2)based on flow chemistry被引量：1
《Chinese Chemical Letters》2023年第5期16-24,共9页Hui Luo Jing Ren Ying Sun Yunlin Liu Feng Zhou Guoyue Shi Jian Zhou 
The financial support from the National Key Research and Development Program of China(No.2020YFA0710200);National Natural Science Foundation of China(No.22171090);the Shanghai Science and Technology Innovation Action Plan(No.20JC1416900);the Fundamental Research Funds for the Central Universities is highly appreciated。
Carbon dioxide(CO_(2))is an attractive C1 building block in chemical synthesis due to its abundance,availability and sustainability.However,the low reactivity and high stability generally limits its transformations un...
关键词：CO_(2)fixation C1 synthon Flow chemistry Cyclic carbonate Carboxylic acid 
TMSCF_(2)Br as both a C1 synthon and a F1 reagent
《Green Synthesis and Catalysis》2022年第4期303-305,共3页Danhua Ge Zhenhua Jia Xuegiang Chu 
We gratefully acknowledge the financial support from the Start-up Grant in Nanjing Tech University(Nos.39837118,39837146);the National Natural Science Foundation of China(No.22001121).
This highlight summarizes a recent development of KF-promoted three-component fluorinationaminocarbonylation reaction of aldehydes,tertiary amines,and TMSCF_(2)Br for the synthesis of structurally importantα-fluoroam...
关键词：TMSCF_(2)Br C1 synthon F1 reagent C-F functionalization Organofluoride 
Simple inorganic base promoted polycyclic construction using mucohalic acid as a C_(3) synthon: synthesis and AIE probe application of benzo[4,5]imidazo[1,2-a]pyridines被引量：1
《Organic Chemistry Frontiers》2022年第4期1127-1136,共10页Kai Yang Zhi-Xi Chen Yong-Jun Zhou Qi Chen Shi-Wei Yu Shi-He Luo Zhao-Yang Wang 
Financial support from the Guangdong Basic and Applied Basic Research Foundation(no.2021A1515012342);the National Natural Science Foundation of China(no.81960883);the Scientific Research Fund of Jiangxi Provincial Education Department(no.GJJ201504);the Guangdong Provincial Science and Technology Project(no.2017A010103016);the Scientific Research Project of Gannan Medical University(no.YB201903)is greatly appreciated.
A transition metal-free and efficient synthesis of fused azapolycycles via a multicomponent reaction has been developed using mucohalic acid as a C_(3) synthon.The reaction promoted by the simple inorganic base K_(2)C...
关键词：INORGANIC promoted SYNTHESIS 
Highly efficient enantioselective synthesis of bispiro[benzofuran-oxindole/benzofuran-chromanone]s through organocatalytic inter-/intramolecular Michael cycloaddition被引量：4
《Chinese Chemical Letters》2020年第2期381-385,共5页Min Zhang Jun-Xin Wang Shun-Qin Chang Xiong-Li Liu Xiong Zuo Ying Zhou 
financial support from the National Nature Science Foundation of China(Nos.81760625,81660576 and81560563);Projects of Guizhou Province(Nos.[2016]5623,JG[2016]06,[2019]1402,[2017]5609 and[2018]5781)。
A quinine-derived thiourea-catalyzed inter-/intramolecular Michael cycloaddition of chromoneoxindole/benzofuranone synthons with 3-substituted methylenebenzofuranones has been established,which constructed enantiomeri...
关键词：Chromone-oxindole SYNTHON Chromone-benzofuranone SYNTHON Inter-/intramolecular Michael CYCLOADDITION Bispiro[benzofuran-oxindole-chromanone] Bispirobenzofuranone 
Ring opening [3+2] cyclization of azaoxyallyl cations with benzo[d]-isoxazoles:Efficient access to 2-hydroxyaryl-oxazolines
《Chinese Chemical Letters》2020年第2期396-400,共5页Yicheng He Chao Pi Yangjie Wu Xiuling Cui 
partial financial support from the Ministry of Science and Technology of China(No.2016YFE0132600);Zhengzhou University。
A selective ring-opening [3+2] cyclization reaction of benzo[d]isoxazoles with 2-bromo-propanamides has been developed.The azaoxyallyl cation intermediates are employed as C^O 3-atom synthon to build oxa-heterocycles ...
关键词：Azaoxyallylic CATIONS RING-OPENING [3+2]Cycloaddition 2-Hydroxyaryl-oxazolines C^O 3-atom SYNTHON 
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