ALIPHATIC

作品数：108被引量：192H指数：6
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相关领域：理学更多>>
相关作者：原小寓于泓王艳潘振宋健刚更多>>
相关机构：中国石油化工集团公司中国石油塔里木油田公司中国石油天然气集团公司中国石化更多>>
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Branched module-modified SN38 prodrug nanoassemblies for improved colorectal cancer therapy:Effectively balance efficacy and safety
《Nano Research》2025年第1期572-585,共14页Qing Wang Shiyi Zuo Shufang Zheng Cuiyun Liu Yaqiao Li Jiayu Guo Danping Wang Shuo Wang Wenjing Wang Bowen Zhang Minglong Huang Xianbao Shi Jin Sun Zhonggui He Bingjun Sun 
gotapproval from the Institutional Animal Ethical Care Committee(IAEC)of Shenyang Pharmaceutical University(ethical code:SYPU-IACUC-2022-0302-010).
The clinical utility of irinotecan is restricted by individual variability in carboxylesterase expression.Direct administration of its active metabolite,7-ethyl-10-hydroxycamptothecin(SN38),presents an appealing alter...
关键词：IRINOTECAN SN38 prodrug nanoassemblies disulfide bonds branched aliphatic chains 
Radical dehydroxymethylative fluorination of aliphatic primary alcohols and diverse functionalization ofα-fluoroimides via BF_(3)·OEt_(2)-catalyzed C-F bond activation
《Chinese Chemical Letters》2025年第1期239-243,共5页Peng Wang Jianjun Wang Ni Song Xin Zhou Ming Li 
financial support from the Marine S&T Fund of Shandong Province for Pilot National Laboratory for Marine Science and Technology(Qingdao)(No.2022QNLM030003-2);the National Natural Science Foundation of China(No.21977088);the National Natural Science Foundation of China-Shandong Joint Fund(No.U1906213)。
Ag_(2)CO_(3)-promoted dehydroxymethylative fluorination of aliphatic alcohols has been achieved with Selectfluor as both oxidant and fluorine source.The reaction involvesβ-fragmentation of primary alkoxy radicals,fol...
关键词：Dehydroxymethylative fluorination Alkoxy radicals β-Fragmentation Silver catalysis C-F Bond activation 
Asymmetric Synthesis of Chiral Aliphaticα-Tertiary Aminonitriles via Organocatalytic Isomerization of Cyanoketimines
《Chinese Journal of Chemistry》2024年第24期3387-3392,共6页Ling Xu Jisheng Luo Li Deng 
the National Natural Science Foundation of China(U22A20389);Foundation of WestlakeUniversity.
Chiralα-tertiary aminonitriles are valuable synthetic intermediates.They are also found in various structures of biologically active molecules.Therefore,numerous reports of catalytic asymmetric synthesis of chiralα-...
关键词：ISOMERIZATION AMINONITRILES Cyanoketimine PROTONATION ORGANOCATALYSIS ENANTIOSELECTIVITY 
Odd-even effects in the structure and properties of aryl-substituted aliphatic self-assembled monolayers
《Nano Research》2024年第5期4231-4243,共13页Piotr Cyganik Andreas Terfort Michael Zharnikov 
supported by BMBF,DFG,NSC Poland,and DAAD through a variety of projects.
Self-assembled monolayers(SAMs)represent an important tool in context of nanofabrication and molecular engineering of surfaces and interfaces.The properties of functional SAMs depend not only on the character of the t...
关键词：self-assembled monolayers molecular films surface and interface engineering odd-even-effects 
Fine-tuning the structure-tolerance-antitumor efficacy axis of prodrug nanoassemblies via branched aliphatic functionalization被引量：1
《Nano Research》2024年第4期2908-2918,共11页Guanting Li Fengli Xia Hongying Xiao Shunzhe Zheng Shuwen Fu Han Qiao Qianhui Jin Xuanbo Zhang Dun Zhou Chutong Tian Jin Sun Zhonggui He Bingjun Sun 
supported by National Natural Science Foundation of China(Nos.82272151,82204318 and 82173766);Doctoral Scientific Research Staring Foundation of Liaoning Province(No.2021-BS-130);General Program of Department of Education of Liaoning Province(No.LJKZ0953);Shenyang Young and Middle-aged Science and Technology Innovation Talent Support Program(No.RC220389).
Small-molecule prodrug nanoassemblies have emerged as efficient antitumor drug delivery systems.However,in the case of camptothecins-based prodrug nanoassemblies,linear aliphatic side chain modification often results ...
关键词：prodrug nanoassembly self-assembly antitumor efficacy TOLERANCE 7-ethyl-10-hydroxycamptothecin(SN_(3)8) 
Impact of Carbon Chain Structures in the Backbone on the Flexibility of Modified Polyarylene Sulfide Resins: Molecular Dynamics Simulations and Mesoscopic Analysis
《Chinese Journal of Polymer Science》2024年第4期544-557,共14页Chi Zhang Rong Liu Jing-Yuan Liu Wen-Wei Jiang 
In the domain of high-performance engineering polymers, the enhancement of mechanical flexibility in poly(phenylene sulfide) (PPS) resins has long posed a significant challenge. A novel molecular structure, designated...
关键词：Molecular dynamics simulations Polyarylene Sulfide Main-chain modifications FLEXIBILITY Aliphatic hexylene chain 
基于电子给体-受体复合物的脂肪烃碳氢键多样性转化
《Science Bulletin》2024年第3期345-353,共9页王泽敏 闫超咸 刘瑞华 李晓伟 戴佳佳 李祥乾 史大永 
supported by the National Key Research and Development Program of China(2022YFC2804105);the Joint Fund of Shandong Natural Science Foundation(ZR2021LSW013);Natural Science Foundation of Shandong Province(ZR2020QB044,ZR2020QH364,ZR2023MH245,and ZR2022QB090);Postdoctoral Science Foundation of China(2020M682157);Qingdao Emerging Industry Cultivation Project in 2023(23-1-4-xxgg-19-nsh);Shandong Provincial Science and Technology SME Innovation Capacity Improvement Project(2022TSGC2204);the National Natural Science Foundation of China(82003787);Postdoctoral Innovation Project of Shandong Province。
The ability to selectively introduce diverse functionality onto hydrocarbons is of substantial value in the synthesis of both small molecules and pharmaceuticals.In this endeavour,as a photocatalyst-and metalfree proc...
关键词：PHOTOREACTION Electron donor-acceptor Aliphatic C-H functionalization Chlorine radicals Gaseous alkanes 
Highly selective extraction of aromatics from aliphatics by using metal chloride-based ionic liquids
《Chinese Journal of Chemical Engineering》2024年第1期222-229,共8页Hui Yu Xiaojia Wu Chuanqi Geng Xinyu Li Chencan Du Zhiyong Zhou Zhongqi Ren 
supported by the National Natural Science Foundation of China(22125802,22078010).
The separation of aromatics from aliphatics is essential for achieving maximum exploitation of oil resources in the petrochemical industry.In this study,a series of metal chloride-based ionic liquids were prepared and...
关键词：Ionic liquid Aromatic hydrocarbon Aliphatic hydrocarbon Extraction 
Olefin Polymerization Behavior of Titanium(IV) Complexes with Fluorinated and Non-fluorinated Aliphatic Phenoxyimine Ligands
《Chinese Journal of Polymer Science》2024年第1期52-62,I0007,共12页Vladislav A.Tuskaev Kasim F.Magomedov Svetlana Ch.Gagieva Dmitry A.Kurmaev Yulia V.Nelyubina Evgenii K.Golubev Maria D.Evseeva Viktor G.Vasil'ev Galina G.Nikiforova Mikhail I.Buzin Vyacheslav S.Bogdanov Boris M.Bulychev 
supported by the Russian Science Foundation (No.22-23-00578);the financial support from the Ministry of Science and Higher Education of the Russian Federation using the equipment of Center for molecular composition studies of INEOS RAS (No.075-00697-22-00);the financial support of the Ministry of Science and Higher Education of the Russian Federation employing the equipment of Center for molecular composition studies of INEOS RAS。
A series of Ti(Ⅳ) dichloride and dialkoxide com plexes with phenoxyimine ligands containing fluorinated and nonfluorinated aliphatic imine fragments have been synthesized.The molecular structures of complexes 1 and 4...
关键词：FI catalysts Titanium(IV) (Co)polymerization Al/Mg co-catalyst Ultra-high molecular weight polyethylene 
Radical Decarboxylative Cyanomethylation of Aliphatic Carboxylic Acids and Uronic Acids via Vinyl Azide Cascade Fragmentation被引量：2
《Chinese Journal of Chemistry》2023年第10期1191-1197,共7页Linhua Xu Qishuai Li Dongwei Li Xin Zhou Ni Song Peng Wang Ming Li 
support from the National Natural Science Foundation of China(Nos.21977088,21672194);the National Natural Science Foundation of China-Shandong Joint Fund(No.U1906213);the Shandong Provincial National Natural Science Foundation(No.ZR2018MB015).
A direct oxidative radical decarboxylative cyanomethylation of carboxylic acids is described using 3-azido-2-methylbut-3-en-2-ol as the carbon-centered radical acceptor.The transformation is applicable to structurally...
关键词：CYANIDES Carboxylic acids Carbohydrates Radical decarboxylation Cyanomethylation 
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