DIRADICAL

作品数：17被引量：10H指数：2
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相关领域：理学更多>>
相关作者：韩莉更多>>
相关机构：山东大学更多>>
相关期刊：《Precision Chemistry》《National Science Review》《Acta Biochimica et Biophysica Sinica》《Nano-Micro Letters》更多>>
相关基金：国家自然科学基金更多>>
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NIR-Ⅱ-activated whole-cell vaccine with ultra-efficient semiconducting diradical oligomers for breast carcinoma growth and metastasis inhibition
《Acta Pharmaceutica Sinica B》2025年第2期1159-1170,共12页Yijian Gao Yachao Zhang Yujie Ma Xiliang Li Yu Wang Huan Chen Yingpeng Wan Zhongming Huang Weimin Liu Pengfei Wang Lidai Wang Chun-Sing Lee Shengliang Li 
upported by the National Natural Science Foundation of China(No.52173135);the Natural Science Foundation of Jiangsu Province(No.BK20231523,China);Jiangsu Specially Appointed Professorship,Leading Talents of Innovation and Entrepreneurship of Gusu(ZXL2022496,China);and the Suzhou Science and Technology Program(SKY2022039,China);Chun-Sing Lee thanks the support of the Research Grants Council of Hong Kong Special Administrative Region,General Research Fund(No.CityU 11300320,11318322,China);Prof.Lidai Wang acknowledges support from the National Natural Science Foundation of China(No.81627805);the Research Grants Council of the Hong Kong Special Administrative Region(21205016,11215817,11101618,China).
High-performance phototheranostics with combined photothermal therapy and photoacoustic imaging have been considered promising approaches for efficient cancer diagnosis and treatment.However,developing phototheranosti...
关键词：NIR-Ⅱ Semiconducting oligomer Photothermal therapy VACCINE Nanoparticles THERANOSTICS Breast carcinoma Immunotherapy 
Cyclooctatetrathiophene Annulated Multicyclic Macrocycles
《CCS Chemistry》2024年第11期2758-2769,共12页Longbin Ren Yi Han Xudong Hou Ya Zou Tianyu Jiao Jishan Wu 
supported financially by the Singapore Ministry of Education(MOE)Academic Research Fund(AcRF)Tier 2 grant(MOE-T2EP10222-0003);the Agency for Science,Technology and Research Manufacturing,Trade,and Connectivity(A*STAR MTC)project,Singapore(M22K2c0083).
The aromaticity and electronic properties of monocyclic or polycyclicπ-conjugated molecules have been widely studied.However,the related research on fullyπ-conjugated multicyclic macrocycles(MMCs)remains limited mai...
关键词：MACROCYCLE AROMATICITY DIRADICAL CYCLOOCTATETRAENE THIOPHENE 
Enhancing stability of diradical polycyclic hydrocarbons via P=O-attaching
《Chinese Chemical Letters》2024年第8期309-313,共5页Jingyuan Yang Xinyu Tian Liuzhong Yuan Yu Liu Yue Wang Chuandong Dou 
supported by Jilin Scientific and Technological Development Program(Nos.20220101054JC,20220201085GX);National Natural Science Foundation of China(Nos.22175074,52373182).
Diradical polycyclic hydrocarbons(PHs)have unique open-shell structures and interesting physical prop-erties.However,owing to high reactivity of unpaired electrons,such open-shell organic diradicaloids are usually les...
关键词：Polycyclic hydrocarbons Open-shell structure Diradical character STABILITY Oxidation activity 
A Stable Open-Shell Conjugated Diradical Polymer with Ultra-High Photothermal Conversion Efficiency for NIR-Ⅱ Photo-Immunotherapy of Metastatic Tumor被引量：1
《Nano-Micro Letters》2024年第2期1-14,共14页Yijian Gao Ying Liu Xiliang Li Hui Wang Yuliang Yang Yu Luo Yingpeng Wan Chun‑sing Lee Shengliang Li Xiao‑Hong Zhang 
The work was financially supported by the National Natural Science Foundation of China(No.52173135,22207024);Jiangsu Specially Appointed Professorship,Leading Talents of Innovation and Entrepreneurship of Gusu(ZXL2022496);the Suzhou Science and Technology Program(SKY2022039).
Massive efforts have been concentrated on the advance of eminent near-infrared(NIR) photothermal materials(PTMs) in the NIR-Ⅱ window(1000–1700 nm), especially organic PTMs because of their intrinsic biological safet...
关键词：NIR-Ⅱconjugated polymer PHOTOTHERMAL RADICAL Nanoparticles Cancer therapy 
A highly efficient open-shell singlet luminescent diradical with strong magnetoluminescence properties被引量：2
《Light(Science & Applications)》2023年第12期2636-2643,共8页Alim Abdurahman Li Shen Jingmin Wang Meiling Niu Ping Li Qiming Peng Jianpu Wang Geyu Lu 
supported by the National Natural Science Foundation of China(Grant Nos.52103210,62022040,51972171,and 61935017);Department of Science and Technology of Jilin Province(20230101363JC);Scientific Research Fund for Doctor of Weifang University(2020BS17);the Science and Technology Huimin Plan of Weifang High-tech Zone(2020KJHM02).
Developing open-shell singlet(OS)diradicals with high luminescent properties and exceptional single-molecule magnetoluminescence(ML)performance is extremely challenging.Herein,we propose a concept to enhance luminesce...
关键词：luminescence LUMINESCENT MAGNETO 
Dual-radical-based molecular anisotropy and synergy effect of semi-conductivity and valence tautomerization in a photoswitchable coordination polymer
《National Science Review》2023年第6期200-214,共15页Jing-Wei Dai Yu-Qin Li Zhao-Yang Li Hai-Tao Zhang Carmen Herrmann Shohei Kumagai Marko Damjanovic Markus Enders Hiroyuki Nojiri Masakazu Morimoto Norihisa Hoshino Tomoyuki Akutagawa Masahiro Yamashita 
the Japan Society for the Promotion of Science for his fellowship(26-14031);the Nankai University for the startup fund for talented young researchers;supported by the National Natural Science Foundation of China(21971124,22275100 and 22150710513);A PhD scholarship from the Beilstein Institut zur Forderung der Chemischen Wissenschaften;state of Baden-Wurttemberg through bw HPC and the German Research Foundation(DFG)through grant no.INST 40/467-1FUGG(JUSTUS cluster);German Research Foundation for the support through project HE5675/6-1(Project ID 420773200)
Organic radicals are widely used as linkers or ligands to synthesize molecular magnetic materials.However,studies regarding the molecular anisotropies of radical-based magnetic materials and their multifunctionalities...
关键词：valence tautomerization charge transfer photo switching DIRADICAL coordination polymer 
Recent Advances of Stable Phenoxyl Diradicals
《Chemical Research in Chinese Universities》2023年第2期170-175,共6页ZHANG Hanjun MIAO Fang LIU Xiaodong WANG Dongsheng ZHENG Yonghao 
National Natural Science Foundation of China(No.52203134);Open Research Fund of State Key Laboratory of Southwestern Chinese Medicine Resources(Chengdu University of Traditional Chinese Medicine),China(No.SKLTCM2022014);partially supported by Grant SCITLAB(No.20012)of Intelligent Terminal Key Laboratory of Sichuan Province and Guangdong Basic,Intelligent Terminal Key Laboratory of Sichuan Province(No.SCITLAB-20013);Applied Basic Research Foundation(No.2021A1515110431).
Organic radicals with unpaired electrons have shown great semiconducting properties with potential applications in the field of organic photodetectors,organic light-emitting diodes and organic spintronics.A major prob...
关键词：PHENOXYL DIRADICAL CONJUGATION STABILITY 
Synthesis and Properties of a Through-Space Interacting Diradicaloid
《Precision Chemistry》2023年第3期183-191,共9页Takuya Kodama Yasukazu Hirao Takashi Kubo 
the JSPS for KAKENHI funding(Grant No.JP21H01918 and JP20K21194);a Grant-in-Aid for Transformative Research Areas(A)“Condensed Conjugation”(JSPS for KAKENHI funding Grant No.JP20H05865)from MEXT,Japan.
Knowledge about electronic structures is important to gain an understanding of the unique functional properties of diradicaloids.In this study,we synthesized and characterized a diradicaloid in which two phenalenyl ra...
关键词：through-space interaction phenalenyl radical singlet diradical diradicaloid antiferromagnetic interaction 
Construction and Functionalization of Highly Strained N-Doped Zigzag Hydrocarbon Belts被引量：1
《CCS Chemistry》2023年第1期117-123,共7页Ming Xie Shuo Tong Mei-Xiang Wang 
We thank the National Natural Science Foundation of China(grant nos.22050005,21732004,and 21821001);the Tsinghua University Initiative Scientific Research Program(grant no.2019Z07L01004)for generous financial support.
Recent years have witnessed breakthroughs in the study of zigzag hydrocarbon belts.However,the synthesis of heterocycle-containing zigzag molecular belts remains very rare and challenging despite their interesting str...
关键词：zigzag molecular belt cyclacene arene[4]pyridine meta-bromination of Nacylaniline palladium-catalyzed C-N bond formation diradical dication salt 
Diradical Character and Controllable Magnetic Properties in Chitin Through Radical Modification被引量：1
《Journal of Donghua University(English Edition)》2022年第1期15-21,共7页KONG Lingqian YANG Hongfang QIAN Zhaohong ZHOU Lianwen ZHANG Mei XU Jing 
Natural Science Foundation of Shandong Province,China(Nos.ZR2016BL13 and ZR2015EQ021);National Natural Science Foundation of China(No.51505065);Foundation for Science and Technology of Shandong Provincial Universities,China(No.J16LC55)。
The parent and radical-modified chitin units are computationally studied and the parent chitin unit possesses closed-shell singlet(CS)state as its ground state.Two radicals(CH_(3)·and CH_(3)CH_(2)·)are chosen to mod...
关键词：radical-modified chitin DIRADICAL magnetic conversion density functional theory(DFT) 
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