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Upgrading ethylene via renewable energy-driven electrocatalysis
《Science China Chemistry》2024年第12期3944-3951,共8页Hanyu Wang Dunfeng Gao Guoxiong Wang Xinhe Bao 
supported by the National Key R&D Program of China(2022YFA1504603);the National Natural Science Foundation of China(22372171,22125205,and 22321002);the Fundamental Research Funds for the Central Universities(20720220008);the Strategic Priority Research Program of the Chinese Academy of Sciences(XDB0600200);the Liaoning Revitalization Talents Program(XLYC2203178);the Liaoning Binhai Laboratory(LBLF-2023-02);the Dalian Institute of Chemical Physics(DICP I202203);the Joint Fund of the Yulin University and the Dalian National Laboratory for Clean Energy(YLUDNL Fund 2022008);the Yanchang Petroleum Group(yc-hw-2023ky-08);the Photon Science Center for Carbon Neutrality。
Ethylene oxide(EO)and ethylene glycol(EG)are two important commodity chemicals and are industrially produced from petroleum-derived ethylene via thermocatalytic processes.The overoxidation of ethylene and the implemen...
关键词：ETHYLENE ethylene oxide ethylene glycol ELECTROCATALYSIS halide mediator selectivity tandem catalysis 
Organo-electroreduction enables arylcarboxylation of styrenes
《Science China Chemistry》2024年第11期3825-3832,共8页Yanwei Wang Qian Wang Zile Zhu Weikang Qi Youai Qiu 
supported by the National Key R&D Program of China (2022YFA1503200);the National Natural Science Foundation of China (22371149, 22301144, 22188101);the Fundamental Research Funds for the Central Universities (63223015);the Frontiers Science Center for New Organic Matter, Nankai University (63181206);Nankai University;the Haihe Laboratory of Sustainable Chemical Transformations for financial support。
Electroreduction offers an alternative to generate high active intermediates from electrophiles(halides, alkenes, etc.) in organic synthesis. However, it still remains challenge to enable the transformations in contro...
关键词：CO_(2)utilization reductive organo-mediator CARBOXYLATION ELECTROREDUCTION aryl halides 
Merging benzotrithiophene covalent organic framework photocatalysis with TEMPO for selective oxidation of organic sulfides
《Science China Chemistry》2023年第11期3290-3296,共7页Fengwei Huang Yuexin Wang Xiaoyun Dong Xianjun Lang 
supported by the National Natural Science Foundation of China (22072108)。
Visible light photocatalysis of covalent organic frameworks(COFs) has made significant progress in recent years. Benzotrithiophene(BTT), a planar, electron-rich building block, turns out to be foundational in assembli...
关键词：sp~2 carbon-conjugated COF electron-rich building blocks visible light hole mediator organic sulfoxides 
Promotion of the oxygen evolution performance of Ni–Fe layered hydroxides via the introduction of a proton-transfer mediator anion被引量：2
《Science China Chemistry》2022年第2期382-390,共9页Wenlong Li Fusheng Li Yilong Zhao Chang Liu Yingzheng Li Hao Yang Ke Fan Peili Zhang Yu Shan Licheng Sun 
financially supported by the National Natural Science Foundation of China(22172011 and 22088102);the K&A Wallenberg Foundation(KAW 2016.0072);Key Laboratory of Bio-based Chemicals of Liaoning Province of China。
Developing efficient catalysts with high durability and activity for the oxygen evolution reaction(OER)is imperative for sustainable energy conversion technologies,including hydrogen generation and CO_(2) reduction,as...
关键词：water splitting Ni Fe–LDH proton-coupled electron transfer proton transfer mediator sulfonate group 
Para-selective borylation of monosubstituted benzenes using a transient mediator被引量：1
《Science China Chemistry》2020年第3期336-340,共5页Jie Wu Zengwei Wang Xiao-Yue Chen Yichen Wu Daoming Wang Qian Peng Peng Wang 
supported by Shanghai Institute of Organic Chemistry,State Key Laboratory of Organometallic Chemistry,the National Natural Science Foundation of China(21890722,21702109,11811530637);the Natural Science Foundation of Tianjin City(18JCYBJC21400);the Fundamental Research Funds for the Central Universities(63191515,63196021,63191523).
Herein,we conceptualized a transient mediator approach that has the capability of para-selective C–H functionalization of monosubstituted aromatics.This approach is enabled by in situ generation of a versatile sulfon...
关键词：para-borylation monosubstituted ARENE TRANSIENT MEDIATOR thianthrenation sulfide DICATION 
Mediated electrochemistry of dimethyl sulfoxide reductase promoted by carbon nanotubes
《Science China Chemistry》2010年第12期2560-2563,共4页BERNHARDT Paul V 
supported by the Australian Research Council(ARC) through Discovery Project Program(DP0880288);the China Scholar-ship Council(CSC)
Mediated electrochemistry of dimethyl sulfoxide reductase from Rhodobacter capsulatus (DMSOR) which is immobilized on a bare glassy carbon (GC) electrode and a carbon nanotube (CNT)-modified GC electrode was studied u...
关键词：DMSO REDUCTASE carbon NANOTUBES ELECTROCHEMISTRY MEDIATOR 
Surface effects of monolayer-protected gold nanoparticles on the redox reactions between ferricyanide and thiosulfate被引量：1
《Science China Chemistry》2005年第5期424-430,共7页LI Di1, SUN Chunyan1, HUANG Yunjie1, LI Jinghong1,2 & CHEN Shaowei3 1. State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China 2. Department of Chemistry, Tsinghua University, Beijing 100084, China 3. Department of Chemistry, University of California, Santa Cruz, Santa Cruz, CA 95064, USA 
financially supported by the National Natural Science Foundation of China(Outstanding Youth Fund Grant No.20125513);a research fellowship from the K.C.Wong Educational Foundation.
Electron transfer through the self-assembled monolayers (SAMs) on gold nanopar-ticles is investigated by using the monolayer protected gold nanoclusters (MPCs) as elec-tron-transfer mediators. 3-Mercaptopropionic acid...
关键词：ELECTRON transfer  three-dimensional self-assembled monolayers  redox reaction  ELECTRON TRANSFER mediator  surface effect. 
LIPOGENESIS STIMULATORY AND INHIBITORY ACTIVITIES OF THE INSULIN MEDIATORS
《Science China Chemistry》1990年第1期60-66,共7页张世荣 乐云 姚文贞 幸兴球 韩锦华 王敬泽 郭宏亮 
Project supported by the National Natural Science Foundation of China.
Incubating plasma membranes prepared from pig liver with varying concentrations of insulin (50—1000 μU/ml) resulted in the release of at least two insulin chemical mediators. One of them was fraction 1 of insulin me...
关键词：INSULIN ANALOGS INSULIN MEDIATOR lipogenesis. 
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