ALKYNE

作品数：113被引量：78H指数：4
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相关领域：理学更多>>
相关作者：张俊良李福伟夏春谷汪文龙朱婧更多>>
相关机构：华东师范大学中山大学厦门大学上海大学更多>>
相关期刊：《Carbon Energy》《Chemical Research in Chinese Universities》《Organic Chemistry Frontiers》《工业催化》更多>>
相关基金：国家自然科学基金国家重点基础研究发展计划广东省自然科学基金中国博士后科学基金更多>>
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Redox-Neutral Nickel-Catalyzed Selective Hydroalkynylation of Internal Alkyne and Its Application in Anticancer Agent Discovery
《Chinese Journal of Chemistry》2024年第24期3317-3323,共7页Weiming Chen Teng Liu Shuqing Li Guangyu Li Gaorong Wu Youjia Gao Zhilin Xu Yitao Wu Xiaopeng Peng Jiuzhong Huang 
supported by the National Natural Science Foundation of China(22361003,82260676);Talent Project of Jiangxi Province(jxsq2019101065);the Jiangxi Provincial Natural Science Foundation(20224BAB216005,20232BAB216131);the Science and Technology Projects of Ganzhou(202101094462,2023PNS26854);The Start-up Fund of Gannan Medical University.
Herein,an unprecedented nickel-catalyzed regioselective hydroalkynylation of unsymmetrical internal alkynes was realized with steric hindered resistance selectivity via the cyano-directing group strategy.Significantly...
关键词：Directing group strategy Hydroalkynylation 1 3-Enynes Dihydroindeno[2 1-c]pyrazole Anti-tumor candidate 
Ni-Catalyzed Enantioselective Difunctionalization of Alkynes to Azepine Derivatives Bearing a Quaternary Center and an Unprotected Imine
《Chinese Journal of Chemistry》2024年第8期873-878,共6页Jian Long Zhiwu Lu Xiao-Lin Li Peng Xue Wen-Bo Liu 
supported by NSFC(22222111,21971198,and 22371215);National Key R&D Program of China(2022YFA1502902);Large-scale Instrument and Equipment Sharing Foundation of Wuhan University.Dr.Zhiwu Lu thanks China Postdoctoral Science Foundation(2022M712458)for the financial support.
Comprehensive Summary,The azepine ring is a prominent structural scaffold in biologically significant molecules. In this study, we present a Ni(II)-catalyzed asymmetric difunctionalization of alkynes, involving interm...
关键词：Nickel Asymmetric catalysis N-HETEROCYCLES Alkyne functionalization Quaternary centers 
Recent Advances in Domino Synthesis of Fused Polycyclic N-Heterocycles Based on Intramolecular Alkyne Hydroamination under Copper Catalysis
《Chinese Journal of Chemistry》2023年第24期3751-3771,共21页Zefeng Jin Guodong Shen Xin Lv 
financial supports from the Natural Science Foundation of Zhejiang Province(LY21B020005);the National Natural Science Foundation of China(21202152).
Fused polycyclic N-heterocycles are very important scaffolds in biomedicinal chemistry and materials science.Intramolecular alkyne hydroamination is a powerful method for the construction of N-heterocycles.In the last...
关键词：Domino reactions Polycyclic N-heterocycles Fused-ring systems Intramolecular hydroamination ALKYNES Copper CYCLIZATION Synthetic methods 
Advances in Transition-Metal-Catalyzed Hydrogermylation of Alkenes and Alkynes
《Chinese Journal of Chemistry》2023年第22期3063-3081,共19页Zungui Zhao Furen Zhang Dongyang Wang Liang Deng 
supported by the National Key Research and Development Program of the Ministry of Science and Technology of China(2021YFA1500203);Natural Science Foundation of China(22201290,22061160464,and 21821002);Shanghai Sailing Program(22YF1458200).
Hydrogermylation of alkenes and alkynes provides a straightforward synthetic route to organogermanium compounds that have been found applications in organic synthesis,medicinal chemistry,and material science.This pape...
关键词：Hydrogermylation ALKENE ALKYNE Diene ALLENE TRANSITION-METAL ORGANOGERMANIUM 
π-Extension of Isoindigos(IIDs)through C—H/N—H Activation and Alkyne Annulation
《Chinese Journal of Chemistry》2023年第20期2589-2596,共8页Kang Wang Liangliang Chen Yan-Ying Huang Liyuan Qin Cheng Li Xi-Sha Zhang Feixian Luo Zheng Duan Guanxin Zhang Deqing Zhang 
This work is supported by the NSFC(Nos.22071254,21790363,22021002,22090021,22171245);X.-S.Zhang is grateful for the funding from Youth Innovation Promotion Association CAs(No.2021032);This work is also supported by the Key Research Program of the Chinese Academy of Sciences(Grant No.121111KYSB20200022);the CAS-Croucher Funding Scheme for Joint Laboratories.
Isoindigo(IID)is widely used as organic dye and conjugated unit in opto-electronic materials.Functionalization of IID to increase its structural complexity is demanding for obtaining diversity properties.Herein,we dev...
关键词：Isoindigo C-H N-H activation Alkyne annulation Opto-electronic function Synthetic methods Functionalized Units 
Activated Internal Alkyne-Based Polymerization
《Chinese Journal of Chemistry》2022年第16期2001-2013,共13页Baixue Li Jia Wang Benzhao He Anjun Qin Ben Zhong Tang 
supported by the National Natural Science Foundation of China(21788102,21901075,22001078);the Natural Science Foundation of Guangdong Province(2016A030312002,2019B030301003);the Innovation and Technology Commission of Hong Kong(ITCCNERC14S01).
As an emerging and efficient polymerization methodology,activated internal alkyne-based polymerization has been considered as a powerful tool for the construction of polymers with diverse architectures and versatile f...
关键词：ALKYNES POLYMERIZATION Polymers Post-functionalization Property and application 
Copper-Catalyzed 1,2,5-Trifunctionalization of Terminal Alkynes Using SR as a Transient Directing Group for Radical Translocation
《Chinese Journal of Chemistry》2022年第14期1667-1673,I0002,共8页Jian Feng Fang Zhang Chenyun Shu Gangguo Zhu 
The first Cu-catalyzed 1,2,5-trifunctionalization of abundant terminal alkynes is realized by merging hydrogen atom transfer and traceless directing strategy with SR as a transient group,delivering highly functionaliz...
关键词：Radical reaction ALKYNE Trifunctionalization Hydrogen atom transfer Copper 
One-Pot Three-Component Synthesis of 2-Methyl-3-aminobenzofurans Using Calcium Carbide as a Concise Solid Alkyne Source被引量：1
《Chinese Journal of Chemistry》2021年第11期2990-2994,共5页Xiaolong Ma Zhiqiang Wang Zhenrong Liu Zheng Li 
The authors thank the National Natural Science Foundation of China(21462038);Key Laboratory of Eco-Environment-Related Polymer Materials of the Ministry of Education of China for their financial support for this work.
A one-pot three-component method for the synthesis of 2-methyl-3-aminobenzofurans using calcium carbide as a concise solid alkyne source,and salicylaldehydes and secondary amines as starting materials is described.Thi...
关键词：CYCLIZATION Multicomponent reactions Synthetic methods Calcium carbide Alkyne source BENZOFURAN 
Seed-mediated Growth of Alloyed Ag-Pd Shells toward Alkyne Semi-hydrogenation Reactions under Mild Conditions
《Chinese Journal of Chemistry》2021年第11期3071-3078,共8页Yuqin Zheng Taixing Tan Cheng Wang 
This work was financially supported by the National Key R&D Program of China(2017YFA0700104);the National Natural Science Foundation of China(21911530255);the State Key Laboratory of Inorganic Synthesis and Preparative Chemistry(2019-6).
Ag@Ag-Pdx core-shell nanocomposites with various Ag/Pd ratio were deposited on Ag nanoplates using a seed growth method.When physically loaded on C3N4,Ag@Ag-Pd0.077/C3N4 with optimized Ag/Pd ratio could accomplish hig...
关键词：NANOSTRUCTURES Alloys Heterogeneous catalysis HYDROGENATION ALKYNES 
Combining Metabolic Alkyne Labeling and Click Chemistry for Secretome Analysis of Serum-Containing Conditioned Medium被引量：1
《Chinese Journal of Chemistry》2021年第7期1843-1848,共6页Jiangnan Zheng Yuan Mao Shun Feng Ruijun Tian 
This work was supported by grants from China State Key Basic Research Program Grants(2016YFA0501403,2016YFA0501404 and 2020YFE0202200);the National Natural Science Foundation of China(31700088);Guangdong Provincial Fund for Distinguished Young Scholars(2019B151502050);Shenzhen Innovation of Science and Technology Commission Grant(JCYJ20170412154126026).
Main observation and conclusion Bioorthogonal click chemistry has emerged as a powerful tool for the specific modification of proteins in complex mixtures.Metabolic labeling of proteins with azide followed by the copp...
关键词：Click chemistry Mass spectrometry PROTEOMICS SECRETOME Metabolic labeling 
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