AMINOCARBONYLATION

作品数：9被引量：3H指数：1
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Regioselective C-C bond cleavage/aminocarbonylation cascade under copper catalysis
《Science China Chemistry》2024年第11期3798-3806,共9页Qi-Chao Shan Yan Zhao Yong Wu Hong-Fei Liu Xin-Hua Duan Li-Na Guo 
supported by the National Natural Science Foundation of China (Nos. 22171220);the Fundamental Research Funds of the Central Universities (No. xtr072022003)。
A regioselective C-C bond cleavage/aminocarbonylation cascade is presented. In recent years, tremendous progress has been made in the alkoxyl radical-mediated C-C bond cleavage of unstrained monocarbocycles. In contra...
关键词：C-C bond cleavage controllable regioselectivity AMINOCARBONYLATION bicyclic alkoxy radical 
Divergent Synthesis of Primary Amides via Modular Dearomative Carbamoylations of Areneπ-Systems
《CCS Chemistry》2024年第8期2066-2074,共9页Chu-Qiao Li Xu Jiang Ming-Yang Wang Wei-Long Zeng Wei Li 
the National Natural Science Foundation of China(grant no.22271251);the Fundamental Research Funds for the Central Universities(grant nos.226-2023-00016,226-2023-00115,and 226-2022-00224).
In sharp contrast to the well researched and well developed aminocarbonylation of alkenes,the dearomative carbamoylation of abundant areneπ-systems has scarcely been studied despite its great potential to enrich the ...
关键词：AMINOCARBONYLATION ARENE CARBAMOYLATION DEAROMATIZATION primary amide 
Controlling Reactivity of Palladium Amides for Selective Carbonylation towards Urea and Oxamide Derivatives
《分子催化（中英文）》2024年第4期297-308,共12页WANG Jin-hui CAO Yan-wei HE Lin 
The National Key Research and Development Program of Ministry of Science and Technology(No.2022YFA1504602);Natural Science Foundation of Jiangsu Province(No.BK20211094);National Natural Science Foundation of China(No.22302214,21972152,U22B20137).
Carbonylation reactions,crucial for carbonyl group incorporation,struggle with the inherent complexity of achieving selective mono-or double-carbonylation on single substrates,often due to competing reaction pathways....
关键词：selectivity control palladium catalysis oxidative carbonylation AMINOCARBONYLATION green reagents 
Photoinduced copper-catalyzed alkoxyl radical-triggered ring-expansion/aminocarbonylation cascade
《Chinese Chemical Letters》2024年第6期331-336,共6页Jing-Qi Tao Shuai Liu Tian-Yu Zhang Hong Xin Xu Yang Xin-Hua Duan Li-Na Guo 
Financial support from the National Natural Science Foundation of China(Nos.21971201,22171220);the Fundamental Research Funds of the Central Universities(No.xtr072022003)。
A photoinduced copper-catalyzed alkoxyl triggered C-C bond cleavage/aminocarbonylation cascade is presented.Through adjusting the structure of alkoxyl radical precursors,functionalized lactones and ketoamides were syn...
关键词：Copper catalysis RING-EXPANSION Aminocarbonylatioin Macrolactones Keto-amides 
Visible-Light-Driven Four-Component Radical Relay Aminocarbonylation of Unactivated Alkenes
《Chinese Journal of Chemistry》2024年第9期990-996,共7页Bin Lu Feng-Shuo Bao Zi-Wei He Wen-Jing Xiao Jia-Rong Chen 
the financial support from the National Natural Science Foundation of China(21971081,22171099,21820102003,91956201,22203034,and 92256301);the Double-Thousand Talents Plan of Jiangxi Province(jxsq2023102004);the Open Research Fund of School of Chemistry and Chemical Engineering,Henan Normal University(2021YB02);and the Program of Introducing Talents of Discipline to Universities of China(111 Program,B17019).
Catalytic four-component radical carbonylation of unactivated alkenes has recently been recognized as a robust protocol for rapid construction of various structurally diverse carbonyl compounds.Given the significance ...
关键词：Visible light Photoredox catalysis Radical aminocarbonylation Multicomponent reaction Carbon monoxide Unactivated alkenes AmidesIReactionmechanisms 
Copper-Catalyzed Hydrogen Production through the Dehydrogenative Coupling of Methanol and Diamine
《Precision Chemistry》2024年第4期138-142,共5页Danyang Cheng Shixiang Yu Meng Wang Ding Ma 
supported by the National Key R&D Program of China(2021YFA1501100);the National Natural Science Foundation of China(22005007);the New Cornerstone Science Foundation,and Liaoning Binhai Laboratory Project(LBLF-202306);the Tencent Foundation through the XPLORER PRIZE.
A hydrogen storage system was developed via heterogeneous catalysis,employing the dehydrogenative coupling of methanol and N,N′-dimethylethylenediamine to efficiently produce high-purity H_(2).In this process,the Cu/...
关键词：methanol reforming hydrogen release AMINOCARBONYLATION dehydrogenative coupling Cu/ZnO/Al_(2)O_(3)catalyst 
Iron-catalyzed hydroaminocarbonylation of alkynes:Selective and efficient synthesis of primaryα,β-unsaturated amides
《Chinese Chemical Letters》2022年第11期4842-4845,共4页Zijun Huang Jia Tang Xiongwei Jiang Tianle Xie Minmin Zhang Donghui Lan Shaofeng Pi Zhengde Tan Bing Yi Yuehui Li 
financial supports from the National Natural Science Foundation of China(Nos.21772035,22022204,22072167,21202206);Natural Science Foundation of Hunan Province(Nos.2021JJ40147)。
α,β-Unsaturated primary amides are important intermediates and building blocks in organic synthesis.Herein,we report a ligand-free iron-catalyzed hydroaminocarbonylation of alkynes using NH_(4)HCO_(3)as the ammonia ...
关键词：Iron-catalyzed ALKYNES Ammonium bicarbonate AMINOCARBONYLATION Linearα β-unsaturated amides 
Palladium-catalyzed tandem Heck/carbonylation/ aminocarbonylation en route to chiral heterocyclic α-ketoamides被引量：1
《Organic Chemistry Frontiers》2022年第4期939-945,共7页Huaanzi Hu Ting Yu Sidi Cheng Jing Li Chunfang Gan Shuang Luo Qiang Zhu 
We gratefully acknowledge the National Natural Science Foundation of China(21772198,21871268,22071250);the Frontier Research Program of Bioland Laboratory(Guangzhou Regenerative Medicine and Health Guangdong Laboratory)(2018GRZ110105017);the Natural Science Foundation of Guangdong Province of China(2020A1515011428);the“BAGUI Scholar”Program of Guangxi Province of China for financial support and Prof.Wenjun Tang at Shanghai institute of Organic Chemistry for providing some of ligands for free.
An unprecedented tandem carbonylation/aminocarbonylation triggered by palladium-catalyzed enantio-selective Heck-type exocyclopalladation delivering chiral heterocyclicα-ketoamides has been developed.The uncommon dou...
关键词：HETEROCYCLIC PALLADIUM catalyzed 
Intermediate formation enabled regioselective access to amide in the Pd-catalyzed reductive aminocarbonylation of olefin with nitroarene被引量：2
《Chinese Journal of Catalysis》2020年第7期1152-1160,共9页Li Yang Lijun Shi Chungu Xia Fuwei Li 
国家重点研发计划(2018YFB1501600);国家自然科学基金(21773271,21972151).
An efficient route for the palladium-catalyzed reductive aminocarbonylation of olefins with nitroarenes was developed using carbon monoxide(CO)as both reductant and carbonyl source,which enables facile access to amide...
关键词：NITROARENES AMIDES N-intermediate AMINOCARBONYLATION Regioselectivity 
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