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Synergistic BrΦnsted/Lewis acid catalyzed atroposelective synthesis of aryl-β-naphthol: 《Chinese Chemical Letters》2025年第1期293-298,共6页Jiajun Lu Zhehui Liao Tongxiang Cao Shifa Zhu; financial support from the National Natural Science Foundation of China(Nos.22071062,22001077 and 22271096);Guangdong Science and Technology Department(Nos.2021A1515012331,2023A1515011001);the Fundamental Research Funds for the Central Universities(No.2022ZYGXZR016);South China University of Technology for start-up funds。; Axially chiral binaphthol have achieved great success in asymmetric catalysis.Compared toα-binaphthol,axially chiral aryl-β-naphthol are far less reported.Here,we report a method of asymmetric catalysis to construct...; 关键词：Synergistic catalysis ATROPISOMERISM Aryl-β-naphthol ENANTIOSELECTIVITY Tandem reaction

Chiral Lewis Base/Achiral Acid Co-Catalyzed Atroposelective Sulfenylation of Pyrrole Derivatives: Construction of C-N Axially Chiral Sulfides被引量：1: 《Chinese Journal of Chemistry》2024年第17期2005-2009,共5页Qin Yang Hui-Yun Luo Deng Zhu Xin-Yu Zhang Hua Ke Zhi-Min Chen; Z.-M.Chen thanks National Natural Science Foundation of China(22071149,21871178);Natural Science Foundation of Shanghai(23ZR1428200);financial support.H.Ke thanks Natural Science Foundation of Jiangxi Province(20202ACBL213005)for financial support.; Chiral BINAM-derived selenide/achiral acid co-catalyzed atroposelective electrophilic sulfenylation of pyrrole derivatives has been realized for the first time.A variety of C-N axially chiral sulfur-containing pyrrole...; 关键词：Electrophilic substitution DESYMMETRIZATION Kinetic resolution ATROPISOMERISM Asymmetric catalysis HETEROCYCLES

Carbene-Catalyzed Asymmetric Ring-Opening Reaction of Biaryl Lactams to Access Axially Chiral Biaryls: 《Chinese Journal of Chemistry》2024年第15期1734-1740,共7页Guanjie Wang Guowei Yuan Chenlong Wei Ye Zhang Haibin Zhu Weiqi Yang Dongping Shi Xiaoxiang Zhang Zhenqian Fu; the Natural Science Foundation of Jiangsu Province(BK20221309);the National Natural Science Foundation of China(21602105).; Axially chiral biaryls represent the most important class of atropisomers,and they widely exist in natural products and biologically active molecules.They also constitute a unique scaffold for chiral ligands and catal...; 关键词：N-Heterocyclic carbene Axially chiral biaryls Organocatalysis Ring-opening reactions Dibenzo cyclic lactams Axially chiral amino acids Amide C-N bond activation ATROPISOMERISM Asymmetric catalysis LACTAMS

An Assembly of Pyrano[3,2-b]indol-2-ones via NHC-Catalyzed[3+3]Annulation of Indolin-3-ones with Ynals: 《Chinese Journal of Chemistry》2024年第13期1487-1492,共6页Xia Wang Shulei Zhang Shao-Jie Wang Hao An Xiaolan Xin Haonan Lin Zhifeng Tu Shenci Lu; We thank the financial support from the Program for Young Talents of Shaanxi Province(5113200043);the Fundamental Research Funds for the Central Universities.; We report herein an unprecedented N-heterocyclic carbene-catalyzed formal[3+3]annulation of ynals with N-Ts indolin-3-ones under the oxidation condition affording the functionalized pyrano[3,2-b]indol-2-ones.The alkyn...; 关键词：N-Heterocyclic carbene ANNULATION ORGANOCATALYSIS ATROPISOMERISM Carbazole Aldehydes HETEROCYCLES Asymmetric catalysis

Asymmetric Two-Component Alkenyl Catellani Reaction for the Construction of C—N Axial Chirality: 《Chinese Journal of Chemistry》2024年第7期699-704,共6页Chenggui Wu Ze-Shui Liu Yong Shang Chang Liu Shuang Deng Hong-Gang Cheng Hengjiang Cong Yinchun Jiao Qianghui Zhou; Herein,we report an asymmetric two-component alkenyl Catellani reaction for the construction of C—N axial chirality through a palladium/chiral norbornene cooperative catalysis and an axial-to-axial chirality transfer...; 关键词：Alkenyl Catellani reaction Asymmetric catalysis ATROPISOMERISM Axial-to-axial chirality transfer HETEROCYCLES

Enantioselective Synthesis of Benzimidazole Atropisomers Featuring a N-N Axis: 《Chinese Journal of Chemistry》2024年第7期711-718,共8页Fang-Bei Ge Qi-Kun Yin Chuan-Jun Lu Xuan Xuan Jia Feng Ren-Rong Liu; supported by Taishan Scholar Youth Expert Program in Shandong Province (tsqn201909096);National Natural Science Foundation of China (22371152);Shandong Provincial Natural Science Foundation Project (ZR2023JQ006,ZR2022MB021);the startup fund from Qingdao University.; Atroposelective synthesis of N-N atropisomers is an emerging area but remains underexplored;in particular,the synthesis of N-N benzimidazole atropisomers is still unprecedented.Herein,the first enantioselective synthe...; 关键词：Asymmetric synthesis ATROPISOMERISM PALLADIUM BENZIMIDAZOLE ANTITUMOR

Preparation of Optically Active 2,2'-Dibromo-6,6'-diiodo-1,1'-biphenyl:A Powerful Precursor for Modular Synthesis of Functionalized Atropisomers: 《Chinese Journal of Chemistry》2023年第24期3515-3520,共6页Yuanyuan Li Longhui Duan Biqiong Hong Zhenhua Gu; financial supports from National Natural Science Foundation of China(92056102);the Natural Science Foundation of Fujian Province(2023J011395).; The widespread applications of atropisomeric compounds have led to an increasing demand for their synthesis.Rather than synthesizing different functionalized atropisomers individually,an attractive alternative is to i...; 关键词：ATROPISOMERISM Asymmetric catalysis Ring-opening reaction CHIRALITY Copper

Synthesis of Axially Chiral Anilides Enabled by a Palladium/Ming-Phos-Catalyzed Desymmetric Sonogashira Reaction被引量：1: 《Chinese Journal of Chemistry》2022年第3期317-322,共6页Bin Yang Junfeng Yang Junliang Zhang; the funding support of NSFC(Nos.22031004,21921003,21901043);Shanghai Municipal Education Commission(No.20212308).; Atropisomeric anilides are one of important C-N axially chiral compounds.Compared with the A/-terminal functionalization to prepare such compounds,C-terminal functionalization strategies have been rarely reported.We d...; 关键词：ATROPISOMERISM Axially chiral anilides SadPhos DESYMMETRIZATION Sonogashira cross-coupling Kinetic resolution

Atroposelective sp3 C—H Coupling for Kinetic Resolution of Thioanilide Atropisomers被引量：2: 《Chinese Journal of Chemistry》2021年第12期3269-3276,共8页Hua-Jie Jiang Rui-Long Geng Jia-Hui Wei Liu-Zhu Gong; We are grateful for the financial support from NSFC(Grant No.21831007).; A highly efficient kinetic resolution of racemic thioanilide atropisomers via C(sp^(3))-H arylation has been achieved by a hybrid palladium catalyst bearing an anionic chiral Co^(Ⅲ)-complex and a phosphoramidite liga...; 关键词：Kinetic resolution C—H activation ATROPISOMERISM Chiral Co^(Ⅲ)-complex PHOSPHORAMIDITE

Atroposelective Construction of Axially Chiral Alkene-lndole Scaffolds via Catalytic Enantioselective Addition Reaction of 3-Alkynyl-2-indolylinethanols被引量：5: 《Chinese Journal of Chemistry》2021年第8期2163-2171,共9页Jing-Yi Wang Meng Sun Xian-Yang Yu Yu-Chen Zhang Wei Tan Feng Shi; We are grateful for financial support from the National Natural Science Foundation of China(Nos.21772069 and 21831007);the Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.KYCX20_2235);the Natural Science Foundation of JSNU(No.19XSRX013)。; Atroposelective construction of axially chiral alkene-heteroaryl scaffolds is highly desired but challenging.In this work,we established an atroposelective construction of axially chiral alkene-indole scaffolds via th...; 关键词：ATROPISOMERISM Axial chirality Asymmetric catalysis INDOLE Nucleophilic addition

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