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AMINATION: 作品数：151被引量：183H指数：7; 导出分析报告; 相关领域：理学更多>>; 相关作者：朱成建王建伟何小伟李江涛钱浩然更多>>; 相关机构：南京大学浙江大学医学院附属第二医院东北电力大学中国科学院大学更多>>; 相关期刊：更多>>; 相关基金：国家自然科学基金中国博士后科学基金王宽诚敎育基金国家重点基础研究发展计划更多>>

Divergent Protein Engineering of Transaminase for the Synthesis of Chiral Rivastigmine and Apremilast Precursors: 《Chinese Journal of Chemistry》2024年第19期2335-2340,共6页Langyu Tang Xinjie Yang Ningning Sun Guojiao Wu Yuzhou Wu Fangrui Zhong; the National Key R&D Program of China(No.2021YFF1200203 to G.W.and 2018YFA0903500 to F.Z.);Hubei Provincial Key R&D program(2021BAA168 to Y.W.);Shen-Zhen Science and Technology Program(JCYJ20220530160805011 to F.Z.);the interdisciplinary research program of Huazhong University of Science and Technology(HUST)(2023JCYJ001 to F.Z.);the China Postdoctoral Science Foundation(2023M741259 to X.Y.)for financial supports.; Comprehensive Summary The implementation of divergent protein engineering on the natural transaminase Vf-ω-TA led to the development of two effective mutants(M2 and M8),enabling the enzymatic synthesis of chiral amin...; 关键词：Asymmetric catalysis Chiral amine Protein engineering Directed evolution BIOCATALYSIS TRANSAMINASE ENANTIOSELECTIVITY Syntheticmethods AMINATION Enzymes

Photoredox-Catalyzed Metal-Free Regio-&Stereoselective C(sp^(2))-H Amination of Enamides with N-Aminopyridium Salts: 《Chinese Journal of Chemistry》2024年第18期2235-2242,共8页Zheng-Bao Qin Kun Ni Li Wang Xiao-Di Wu Yu Zhang Kai Zhao; the financial support from the National Natural Science Foundation of China(21801129,22078153 and 22378201);National Key Research and Development Program of China(2022YFB3805603);Natural Science Research Projects in Jiangsu Higher Education Institutions(18KJB150018);Nanjing Tech University(Start-up Grant Nos.39837137,39837101 and 3827401739)for financial support.; A visible-light-induced photoredox-catalyzed regioselective and stereoselective C(sp')-H amination of enamides with bench-stable and A visible-light-induced photoredox-catalyzed regioselective and stereoselective C(sp...; 关键词：ENAMIDES AMINATION Photoredox catalysis REGIOSELECTIVE STEREOSELECTIVE METAL-FREE

Atroposelective Synthesis of 2-Arylindoles via Chiral Phosphoric Acid-Catalyzed Direct Amination of Indoles被引量：1: 《Chinese Journal of Chemistry》2024年第7期731-735,共5页Wen Bao Ye-Hui Chen Yu-Wei Liu Shao-Hua Xiang Bin Tan; support from the National Key R&D Program of China (2022YFA1503703,2021YFF0701604);the National Natural Science Foundation of China (21825105,22231004,22271135);Guangdong Innovative Program (2019BT02Y335);Shenzhen Science and Technology Program (KQTD20210811090112004,JCYJ20210324120205016,JCYJ20210324105005015).; Indole-based atropisomers are a very important class of axially chiral compounds.However,the atroposelective synthesis of axially chiral 2-arylindole remains largely unexplored.In this study,we report the successful s...; 关键词：Chiral phosphoric acid Quinonediimines Direct amination Nucleophilic addition Asymmetric catalysis Enantioselectivity Axially chiral 2-arylindole Atroposelective synthesis

Decarboxylative Amination with Nitroarenes via Synergistic Catalysis: 《Chinese Journal of Chemistry》2024年第4期351-355,共5页Meiling Ding Sitian Zhou Shunruo Yao Chengjian Zhu Weipeng Li Jin Xie; National Key Research and Development Program of China(2022YFA1503200,2021YFC2101901);the National Natural Science Foundation of China(22122103,22101130,22001117,21971108,22271144);Fundamental Research Funds for the Central Universities(020514380304,020514380252,020514380272)for financial support.; In this paper,we have developed a decarboxylative amination of carboxylic acids with nitroarenes for the synthesis of secondary amines.The protocol is performed at mild conditions without the use of noble metals as ca...; 关键词：NITROARENES AMINES Synergistic catalysis Carboxylic acids Radical alkylation AMINATION PHOTOCATALYSIS Steric hindrance

Synthesis of 2,3-Diaminoindoles via a Copper-Iodine Co-catalytic Strategy: 《Chinese Journal of Chemistry》2023年第24期3567-3572,共6页Wenhua Yu Yingying Zhang Xiaoxiang Zhang Xiaoting Gu Xirui Qing Wanxing Wei Zhuan Zhang Guanghua Li Taoyuan Liang; the National Natural Science Foundation of China(22201048);the Natural Science Foundation of Guangxi Province(2022GXNSFBA035480);the Specific Research Project of Guangxi for Research Bases and Talents(2022AC21099);the Start-up Fund of Guangxi University(A3040051013)for financial support.; A one-pot synthesis of vicinal diamines using indoles,azoles and phenothiazines in a tandem multi-component reaction is developed.The utilization of a copper-iodine co-catalytic system enables the generation of a dive...; 关键词：INDOLES Tandem dual C—H amination Vicinal diamines Copper-iodine co-catalysis Multi-component reaction

Selective Carbon-Carbon Bond Amination with Redox-Active Aminating Reagents:A Direct Approach to Anilines: 《Chinese Journal of Chemistry》2023年第18期2408-2408,共1页Xu Qiu Yachong Wang Lingyu Su Rui Jin Song Song Qixue qin Junhua Li Baoning Zong Ning Jiao; The structure of Montelukast-derivatives(12)in Table 2 and the structure of its product 25 in page s24 are wrong,and they should be Montelukast-derivatives(12)methyl(R,E)-2-(1-(1-(3-(2-(7-chloroquinolin-2-yl)vinyl)phe...; 关键词：VINYL PHENYL Redox

Enantioselective and Enantioconvergent Iron-Catalyzed C(sp^(3))-H Aminations to Chiral 2-Imidazolidinones被引量：1: 《Chinese Journal of Chemistry》2023年第17期2065-2070,共6页Tianjiao Cui Chen-Xi Ye Jordan Thelemann Daniel Jenisch Eric Meggers; the European Research Council(ERC)under the European Union's Horizon 2020 research and innovation programme(grant agreement No.883212).; Comprehensive Summary Enantioselective or enantioconvergent iron-catalyzed ring-closing C(sp^(3))-H aminations of N-aroyloxyurea through intermediate iron nitrene species provide chiral 2-imidazolidinones in up to 99%...; 关键词：Iron Asymmetric catalysis C-H activation AMINATION NITRENES HETEROCYCLES

[3+2]Cycloaddition of Vinyl Cyclopropane and Hydroxylamines via Isocynate Intermediate toγ-Lactams被引量：1: 《Chinese Journal of Chemistry》2023年第16期1937-1942,共6页Xiaobing Huang Jingxun Yu Xinjun Luan; the National Natural Science Foundation of China(21925108,21901203,21901204)for financial support.; Comprehensive Summary A general and efficient strategy for the synthesis ofγ-lactams has been reported.The hydroxylamines form Lossen rearrangement products of electron-deficient group migration with base and then un...; 关键词：γ-Lactams HYDROXYLAMINES VinyI cyclopropane PD-CATALYZED [3+2]cycloaddition AMINATION Insertion Ring expansion

Visible Light-Driven Catalyst-Free Amination of Indoles Initiated by Electron Donor-Acceptor Complexes被引量：1: 《Chinese Journal of Chemistry》2023年第12期1485-1490,共6页Jiahong Sui Zhonglie Yang Shuangqiao Li Xueqin Chen Xiaobin Zhang Qing Shen Hezhong Jiang Jiahong Li; financial support from the National Natural Science Foundation of China(Grant Nos.21901216 and 82074003,82174083);the Funds of Sichuan Science and Technology Program(23NSFSC0862,2021YFSY0041,2021YFH0064 and 2021ZHFP0032);the Opening subject under KF-202204 in the State Key Laboratory of Pharmaceutical Biotechnology,Nanjing University,China,the Fund of Science and Technology Agency of Chengdu(2019-YF09-00049-SN);the research project of the Administration of Traditional Chinese Medicine of Sichuan(2021MS110);the Open Project Program of Irradiation Preservation Technology Key Laboratory of Sichuan Province,Sichuan Institute of Atomic Energy(No.FZBC2020002);the Fundamental Research Funds for the Central Universities(2682020ZT85).; The visible light-driven C2 or C3 amination of indoles without any additives was initiated via electron donor-acceptor (EDA) complex formed by indole and N-aminopyridinium salt.This method was compatible with a wide r...; 关键词：PHOTOCHEMISTRY AMINATION C-N bond formation Green chemistry N-HETEROCYCLES Donor-acceptor systems

Kinetic Resolution of 1,2-Diamines via Organocatalyzed Asymmetric Electrophilic Aminations of Anilines被引量：2: 《Chinese Journal of Chemistry》2022年第14期1674-1680,共7页Jinglei Xie Zheng Guo Wei Liu Dekun Zhang Yu-Peng He Xiaoyu Yang; NSFC(Grant No.22171186) and ShanghaiTech University start-up funding for financial support;the support from Analytical Instrumentation Center(contract no.SPST-AIC10112914),SPST。; An efficient kinetic resolution(KR)protocol for 1,2-diamines has been developed through asymmetric electrophilic aminations of anilines enabled by chiral phosphoric acid catalysis.A wide array of substituted 1,2-diami...; 关键词：Asymmetric catalysis 1 2-Diamines Kinetic resolution Chiral phosphoric acids AMINATION

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